Molecular orbital treatment of pyridine 1-nitroimide predicts well the site of protonation, u.v. spectrum, and reactivity. The ring resists electrophillic attack but α-protons are readily replaced by deuterium in the presence of base. The mass spectral framentation is elucidated.
J. Arriau, A. Dargelos, J. Epsztajn, A. R. Katritzky, E. Lunt, J. W. Mitchell, S. Q. A. Rizvi and G. Roch, J. Chem. Soc., Perkin Trans. 2, 1976, 1245 DOI: 10.1039/P29760001245
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