Departures from physical reality in the phase equilibrium and gas-liquid properties predicted for binary mixtures by the two- and three-fluid models are reported, and shown to derive from the averaging for the (p, V) isotherms implied in the models.
C. P. Hicks, J. Chem. Soc., Faraday Trans. 2, 1976, 72, 423 DOI: 10.1039/F29767200423
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