Intensity beats have been observed in the pure rotational Raman spectra of several near prolate asymmetric top molecules. Comparison of the observed spectra with computer simulated ones allows, from a knowledge of A0 and B0, the determination of both B0 and C0 for butadiene: B0= 0.148 7 ± 0.000 2 cm–1, C0= 0.133 9 ± 0.000 2 cm–1.
G. W. Hills and W. J. Jones, J. Chem. Soc., Faraday Trans. 2, 1975, 71, 835 DOI: 10.1039/F29757100835
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