E.s.r. spectra of nitroxide radicals with S=½, I= 1 have been simulated for reorientation rates that are insufficient to achieve rapid tumbling. The radical is assumed to be attached to a rod-shaped molecule which is reorienting by strong collisions; these preferentially rotate the molecule about its long axis, giving anisotropic reorientation.
J. E. Benton and R. M. Lynden-Bell, J. Chem. Soc., Faraday Trans. 2, 1975, 71, 807 DOI: 10.1039/F29757100807
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