It is shown that the ability of some hydrides, trans-MHX(PR3)2, where M = Ni or Pd, to act as catalysts for butadiene oligomerisation depends markedly both on the nature of the substituent X and on the solvent. The cationic hydrides [PdH(PR3)(dppe)]+PF6–, where R = cyclohexyl or Pri have been prepared and their reactions with butadiene explored.
M. L. H. Green and H. Munakata, J. Chem. Soc., Dalton Trans., 1974, 269 DOI: 10.1039/DT9740000269
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