It is shown that the expression for the primary medium effect obtained by the application of macroscopic equilibrium thermodynamic expressions for a multi-component fluid in an electric field is, when valid, entirely equivalent to that based on the Kirkwood-Buff theory of solutions.
D. G. Hall, J. Chem. Soc., Faraday Trans. 2, 1973, 69, 975 DOI: 10.1039/F29736900975
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