Tetrasulphur dinitride, as prepared by published methods, is a single substance and not a mixture of isomers. Its dipole moment, 14N n.m.r. spectrum, mass spectrum, electronic spectrum, i.r. spectrum, and Raman spectrum have been determined. This physical evidence shows that the compound has a cyclic structure with the nitrogen atoms in the 1,3-positions.
J. Nelson and H. G. Heal, J. Chem. Soc. A, 1971, 136 DOI: 10.1039/J19710000136
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