The vitamin B12 model compounds trans-[RCo(tim)X]Y and trans-[RCo(cr)X]Y can be reduced to neutral alkylcobalt(I) complexes of a new type, which are readily oxidatively alkylated at the cobalt atom to yield trans-dialkylcobalt(III) derivatives.
K. Farmery and D. H. Busch, J. Chem. Soc. D, 1970, 1091 DOI: 10.1039/C29700001091
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