Assignment of the high-resolution photoelectron spectrum of BF3 shows that the highest occupied orbital is of π(e″) type, rather than σ(a2′ or e′) as predicted, and that one of the ionic excited states is probably distorted.
P. J. Bassett and D. R. Lloyd, J. Chem. Soc. D, 1970, 36 DOI: 10.1039/C29700000036
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