The relative importance of charge transfer states arising by excitation of electrons from π and from nitrogen non-bonding orbitals to the lowest vacant s-orbital of the alkali metal as mechanisms producing metal hyperfine splitting in the electron spin resonance spectra of pyrazine-alkali metal ion pairs is discussed using molecular orbital theory.
N. M. Atherton, Trans. Faraday Soc., 1966, 62, 1707 DOI: 10.1039/TF9666201707
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