The properties of the yellow compound Fepy4(NCS)2 and of its so-called “black isomer” have been examined by a variety of physical methods. We conclude that the yellow form has a trans configuration, but that the “black” modification is really the yellow form containing a small, and probably variable, amount of some iron(III) derivative. Some properties of the complex Fepy3(NCS)3 are reported.
C. D. Burbridge, M. J. Cleare and D. M. L. Goodgame, J. Chem. Soc. A, 1966, 1698 DOI: 10.1039/J19660001698
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