Toughening self-healable and recyclable PDMS supramolecular elastomers through an end-capping agent and a metallic crosslinker

Rou-Han Lai, Yi-An Chen, Chung-Ying Chou, Hung-Yi Huang, Wassana Mongkonkan, Chia-An Chiu, Yan-Heng Chen, Min-Han Yu, Chi-Chang Hu, Siriporn Jungsuttiwong and Ho-Hsiu Chou

J. Mater. Chem. A, 2025, 13, 14588
DOI: 10.1039/D4TA08955C

Self-crosslinking pyrimidine siloxanes with tunable mechanical and adhesive properties

Manman Wu, Xinyi Han, Rui Bao, Xiangyu Ma, Kaili Zhao, Jiale Yang, Xinyao Yang, Jiyuan Han, Xiao Cheng and Chuanjian Zhou

Polym. Chem., 2025, 16, 4433
DOI: 10.1039/D5PY00616C

A room-temperature self-healing and mechanically robust siloxane elastomer via synergistic complexation and cation–π interactions for high-performance electromagnetic interference shielding

Suting Chen, Ziyi Liu, Tian Qiu, Ting Zhang, Chaoqun Ma, Dongjin Xie, Tengning Ma, Li Yang, Guanjun Chang and Ying Huang

J. Mater. Chem. A, 2025, 13, 26310
DOI: 10.1039/D5TA03799A

Development of a coarse-grained molecular dynamics model for poly(dimethyl-co-diphenyl)siloxane

Weikang Xian, Amitesh Maiti, Andrew P. Saab and Ying Li

Soft Matter, 2024, 20, 8480
DOI: 10.1039/D4SM00875H

Developing mechanically robust, self-healable, and antibacterial poly(dimethylsiloxane) elastomers through the introduction of metal-polyphenol networks

Yan Huang, Qingqing Hao, Hao Chen, Jianyu Liu, Jie Liu, Yusheng Qin, Zhengfeng Ma, Zhuhui Qiao, Zhirong Xin and Chunyang Bao

Polym. Chem., 2025, 16, 3570
DOI: 10.1039/D5PY00629E

Tough silicone-based elastomers enhanced by synergistic Zn(ii)–carboxylate interactions and weak hydrogen bonds between incompatible soft segments

Yangjiao Han, Kaixin Xi, Chengshu Zhang, Wenpin Wang and Zhibo Li

J. Mater. Chem. A, 2025, 13, 13305
DOI: 10.1039/D5TA01214G

Hydrogen-bonded polymeric materials with high mechanical properties and high self-healing capacity

Jianglong Li, Xiaoyu Du, Aofei Zhang, Jianlong Wen, Lang Shuai, Sumin Li, Maiyong Zhu and Yijing Nie

Mater. Chem. Front., 2024, 8, 3828
DOI: 10.1039/D4QM00472H

High-strength, self-healing conductive polyurethane with covalent crosslinking and reversible dynamic bonds for multifunctional strain sensors

Zhecheng Hu, Changsheng Wang, Xiwei Xu, Ziqian Wang, Yuxuan Xie, Zequan Li and Wei Gao

J. Mater. Chem. C, 2025, 13, 8990
DOI: 10.1039/D5TC00470E

Multiple hierarchical dynamic interactions enabled a robust, stretchable and room temperature self-healing elastomer

Jianfeng Fan, Xinqin Zhou and Yukun Chen

Polym. Chem., 2023, 14, 2117
DOI: 10.1039/D3PY00187C

High toughness, healable, self-cleaning polydimethylsiloxane elastomers with “rigid-while-flexible” mutual network structure

Xing Yang, Jiawen Ren, Baoquan Wan, Sichen Qin, Qian Wang, Wenjie Huang, Jinghui Gao, Bing Xia and Jun-Wei Zha

Mater. Horiz., 2024, 11, 5058
DOI: 10.1039/D4MH00409D

Enhanced Electro-Actuation and Self-Healing Properties of Dielectric Elastomers by Introducing Ultrafine BaTiO3 and Semi-Interpenetrating Macromolecules

Haotong Guo, Chuying Zhang, Na Zhang, Liming Jin, Yanfei Gao, Jinbo Bai and Hang Zhao

ACS Appl. Polym. Mater., 2025, 7, 680
DOI: 10.1021/acsapm.4c03003

Stabilize and Reinforce Hydrogen-Bonded Polymer Complex Elastic Fiber by Catechol Chemistry and Coordination

Ze-Xin Liu, De-Zhong Liu, Cai-Hong Zhang, Wei-Jie Wang, Hao Huang and Shu-Guang Yang

Chin J Polym Sci, 2023, 41, 1846
DOI: 10.1007/s10118-023-2992-5

Designing Strong yet Tough, Multifunctional and Printable Dynamic Cross‐Linking Waterborne Polyurethane for Customizable Smart Soft Devices

Xingyuan Lu, Hongqiu Wei, Ping Zhang, An Wei, Siying Zhao, Qian Wang, Jupen Liu and You Yu

Adv Funct Materials, 2025, 35
DOI: 10.1002/adfm.202502720

Ultra-tough and stress-free two-way shape memory polyurethane induced by polymer segment “spring”

Yutong Guo, Yujie Chen, Qili Yu, Hezhou Liu, Hua Li and Yinxian Yu

Chemical Engineering Journal, 2023, 470, 144212
DOI: 10.1016/j.cej.2023.144212

Ultralow-Temperature-Resistant Poly(ethylfluorophenylsiloxane) Elastomers Synthesized by Postpolymerization Macromolecular Chain Exchange Reaction

Linyu Li, Hang Zheng, Zhu Xia, Zhanwei Feng, Xiaoning Hou, Jianyun He, Yuanwei Yan, Zhen Niu and Chenxi Bai

Macromolecules, 2025, 58, 4746
DOI: 10.1021/acs.macromol.5c00009

Highly stretchable and room-temperature self-healing sheath-core structured composite fibers for ultrasensitive strain sensing and visual thermal management

Zhonglei Ma, Yan Zhang, Ruochu Jiang, Liang Shao, Jinan Cao, Hao Guo and Guangcheng Zhang

Composites Science and Technology, 2024, 248, 110460
DOI: 10.1016/j.compscitech.2024.110460

Rosin-based self-healing functionalized composites with two-dimensional polyamide for antimicrobial and anticorrosion coatings

Yuedong Xing, Liwei Lu, Jiongchao Li, Jianben Xu and Faai Zhang

International Journal of Biological Macromolecules, 2024, 273, 133152
DOI: 10.1016/j.ijbiomac.2024.133152

Ultra‐Dense Bottlebrush Dynamic Phase Change Polymer Networks with Ultra‐High Latent Heat and Adaptive Electrically Conductive for Intelligent Thermal Storage and Device

Yanyun Li, Jiahao Ma, Qiguang Liu, Zhihao Zhang, Tiancheng Wang, Junying Zhang and Jue Cheng

Adv Funct Materials, 2025
DOI: 10.1002/adfm.202519513

Room-Temperature Self-Healable Glassy Semicrystalline Polymers via Ionic Aggregations

Pengxiang Si, Bowen Zhu, Yuhang Tong, Zhu Long, Yun Wu and Dan Zhang

Macromolecules, 2024, 57, 11705
DOI: 10.1021/acs.macromol.4c02387

High strength, recyclable, durable polydimethylsiloxanes based on carboxylic acid aromatic disulfides with highly efficient room-temperature self-healing

Hao Dong, Xing Yang, Wenjie Huang, Jiefeng Gao and Jun-wei Zha

Polymer, 2025, 320, 128125
DOI: 10.1016/j.polymer.2025.128125

Dynamic crosslinked elastomers and rubbers

Jing Bai, Baochun Guo, Ming Tian, Fei Chen and Liqun Zhang

Progress in Materials Science, 2026, 155, 101536
DOI: 10.1016/j.pmatsci.2025.101536

Highly Stretchable and Self-Healable Tough Polymer Elastomer through Dy3+ and Cu2+ Coordination Cross-Linking

Xiuyu Huang, Aofei Zhang, Qiuli Tan, Kai Gou, Yang Chen, Yijing Nie and Gengsheng Weng

Macromolecules, 2024, 57, 963
DOI: 10.1021/acs.macromol.3c02347

Recent advancements in wearable self-healing polysiloxane materials and wearable sensors

Tao Liu, Tian Wang, Shuai Zhang and Bo Jiang

Wearable Electronics, 2025, 2, 40
DOI: 10.1016/j.wees.2024.12.002

The Mechanical and Rheological Properties of Polydimethylsiloxane Elastomers Prepared by a Hydrosilylation Reaction

Abdulraheem A. Alrefai, Alessandra Petroli, Yuan Xu, Steve J. Bull and Mark Geoghegan

J of Applied Polymer Sci, 2025
DOI: 10.1002/app.57953

Room temperature self-healable and recyclable polyurethanes with tunable mechanical properties by integrating dual dynamic units of hydrogen bonding and metal−lysine coordination bonds

Zhi Li, Xingshuang Lv, Xunling Zhu and Xiaohui Fu

European Polymer Journal, 2025, 234, 114015
DOI: 10.1016/j.eurpolymj.2025.114015

Light-activated cellulose nanocrystals/fluorinated polyacrylate-based waterborne coating: Facile preparation, mechanical and self-healing behavior

Hong Li, Jianhua Zhou, Jiarui Yu and Jiaojiao Zhao

International Journal of Biological Macromolecules, 2023, 249, 126062
DOI: 10.1016/j.ijbiomac.2023.126062

Self-Healing Silicone Materials: Looking Back and Moving Forward

Konstantin V. Deriabin, Sofia S. Filippova and Regina M. Islamova

Biomimetics, 2023, 8, 286
DOI: 10.3390/biomimetics8030286

Tough and self-healing linear polydimethylsiloxane elastomer with multiple hydrogen bonds for high-performance piezoresistive pressure sensor

Hongtao Zhu, Han Lu, Junhuang Xu, Xuejun Lai, Hongqiang Li, Xingrong Zeng, Xiangrong Wu and Hong Liu

Applied Materials Today, 2024, 40, 102411
DOI: 10.1016/j.apmt.2024.102411

Facial fabrication of self‐healing natural rubber foam based on zinc thiolate ionic networks

Noor Aishatun Majid, Abdul Rehman, Noor Faezah Mohd Sani, Nabil Hayeemasae, Hanafi Ismail, Mimi Syahira Masraff and Raa Khimi Shuib

J of Applied Polymer Sci, 2024, 141
DOI: 10.1002/app.55280

High-Molecular-Weight Poly(fluorophenylsiloxane) Elastomers via Postpolymerization Macromolecular Chain Exchange Reaction for Optimized Comprehensive Properties

Linyu Li, Zhen Niu, Hang Zheng, Zhanwei Feng, Xiaoning Hou, Weifeng Fan, Jianyun He and Chenxi Bai

ACS Appl. Polym. Mater., 2025, 7, 15111
DOI: 10.1021/acsapm.5c03360

Highly Durable Silicone‐Based Elastomers Achieved Through the Synergy of Bi‐Incompatible Soft Segments and Multi‐Scale Hydrogen Bonds

Wei Zheng, Chengshu Zhang, Yangjiao Han, Wenpin Wang and Zhibo Li

Small, 2024, 20
DOI: 10.1002/smll.202402124

Recent achievements and applications of photothermal self-healing coatings: A review

Huimeng Feng, Tong Wang, Lin Cao, Yanan Pu, Zhipeng Zhao and Shougang Chen

Progress in Organic Coatings, 2024, 187, 108153
DOI: 10.1016/j.porgcoat.2023.108153

Supramolecular Ionic Gels with High Elasticity and Self-Healing Based on Polymeric Deep Eutectic Solvent for 3D-Printable Soft Sensors

Jun Hu, Xin Yao, Tianqiang Li, Xiaojie Li, Wei Wei and Jingcheng Liu

ACS Appl. Polym. Mater., 2023, 5, 9650
DOI: 10.1021/acsapm.3c02114

A hybrid reversible crosslinked polysiloxane elastomer with high toughness and recyclability

Fang Wang, Chengshu Zhang, Yangjiao Han, Gang Yi, Zhengnan Mao, Juan Li, Zhongcheng Li and Wenpin Wang

Journal of Polymer Science, 2024, 62, 2147
DOI: 10.1002/pol.20240019

Secondary Network Formation in Epoxidized Natural Rubber with Alternative Curatives

Alexandra Shakun, Noora Kemppainen and Essi Sarlin

ACS Omega, 2024
DOI: 10.1021/acsomega.4c03271

Renewable Elastomers of Ethylene with Propylene Based on Triple Reversible Cross-Linking Sites

Yicong Wang, Peiyi Cheng, Shu Zhang and Yixian Wu

Macromolecules, 2025, 58, 7301
DOI: 10.1021/acs.macromol.5c00235

Non-isocyanate route of biomimetic hierarchical hydrogen-bonding elastomers with solvent and temperature-assisted healability via structural functional region engineering for electronic skin applications

Xuedong Lv, Weidi Sun, Chen Sheng, Gouming Liu, Yi Liu, Yongjun Zhang and Liuchun Zheng

Chemical Engineering Journal, 2025, 524, 168685
DOI: 10.1016/j.cej.2025.168685

A ENR-based conductive film integrating electricity-triggered self-healing, damage detection and high sensitivity for flexible sensors

Lingli Kong, Yunpeng Yang, Zihao Lin, Bai Huang, Lusheng Liao, Yueqiong Wang and Chuanhui Xu

Chemical Engineering Journal, 2024, 479, 147624
DOI: 10.1016/j.cej.2023.147624

A super‐stretched self‐healing silicone elastomer based on high molecular weight polydimethylsiloxanes through intermolecular quadruple hydrogen bonding

Yue Lang, Wei Zheng, Wenpin Wang and Zhibo Li

Polymers for Advanced Techs, 2023, 34, 2823
DOI: 10.1002/pat.6107

Self-assembly of modified cellulose nanocrystals on flexible fabric via hydrophobic force induction for versatile applications

Fan Xiang, Manman Zhao, Xiaoyue Yang and Zhanxiong Li

Progress in Organic Coatings, 2024, 190, 108406
DOI: 10.1016/j.porgcoat.2024.108406

Designing Highly Entangled, Homogeneous, and Low-Defect Networks for High-Performance Rubbers

Lingmin Kong, Junqi Zhang, Shaoqi Huang, Rongchun Zhang, Jiaming Li, Zhengtian Xie and Jinrong Wu

Macromolecules, 2025, 58, 3109
DOI: 10.1021/acs.macromol.4c03133