Issue 23, 2023

Heterostructured 2D material-based electro-/photo-catalysts for water splitting

Abstract

We provide a comprehensive overview of the recent developments in the field of two-dimensional (2D) materials for energy conversion and storage applications. The focus of this review is the electronic structure tuning of 2D materials such as carbon/graphene, metal dichalcogenides, metal oxides/hydroxides, and MXenes for the hydrogen evolution reaction. This review begins with presenting a systematic classification, controllable synthesis, and formation mechanism of 2D nanomaterials. It then discusses the strategies for tuning the electronic structure of 2D nanomaterials and their impact on electro-/photo-catalytic properties, particularly through composite and heterostructure formation (0D/2D, 1D/2D, and 2D/2D). The latest advances in the development of electro-/photo-catalysts with novel nanosheet structures and compositions are discussed in detail. The correlation between the electronic nature; activity; and the shape, size, composition and synthesis methods of these materials is summarized. Finally, this review concludes with perspectives on future challenges and directions for research in this field.

Graphical abstract: Heterostructured 2D material-based electro-/photo-catalysts for water splitting

Article information

Article type
Review Article
Submitted
16 Mai 2023
Accepted
28 Aug 2023
First published
05 Sep 2023

Mater. Chem. Front., 2023,7, 6154-6187

Heterostructured 2D material-based electro-/photo-catalysts for water splitting

E. Heo, S. Lee and H. Yoon, Mater. Chem. Front., 2023, 7, 6154 DOI: 10.1039/D3QM00566F

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