Issue 7, 2024

Solvent selection based on a conceptual process design by combining cost evaluation and life cycle assessments for developing new reaction pathways

Abstract

Solvents have a significant impact on the efficiency and performance of chemical production. A large amount of solvent disposed after chemical production negatively impacts the environment and the economy. This study presents a solvent selection method based on a conceptual process design, which includes solvent processes used in chemical synthesis and waste solvent treatment. The proposed method is demonstrated with Suzuki–Miyaura coupling as a model reaction. The results show that solvent recycling costs and CO2 emissions were lower than those observed for incineration. Importantly, if the appropriate solvent is selected, the cost and CO2 emissions can be reduced by up to 67% and 70%, respectively, even with similar yields in the reaction. These results suggest that solvent selection combined with conceptual process design is the key to developing sustainable chemical production.

Graphical abstract: Solvent selection based on a conceptual process design by combining cost evaluation and life cycle assessments for developing new reaction pathways

Supplementary files

Article information

Article type
Paper
Submitted
06 ное 2023
Accepted
22 яну 2024
First published
19 фев 2024

Green Chem., 2024,26, 3758-3766

Solvent selection based on a conceptual process design by combining cost evaluation and life cycle assessments for developing new reaction pathways

T. Yamaki, T. T. H. Nguyen, N. Hara, S. Taniguchi and S. Kataoka, Green Chem., 2024, 26, 3758 DOI: 10.1039/D3GC04293F

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