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Abstract | Cited by

Tailoring defects in metal–organic frameworks is important for enhancing sorption and reaction properties. Defects in UiO-66 have been characterized for the first time by using water adsorption measurements. We found that the defect-induced hydrophilicity, quantitatively expressed by the Henry constant and the saturation water uptake, correlates well with the catalytic performance in the cyanosilylation of benzaldehyde.

Graphical abstract: Using water adsorption measurements to access the chemistry of defects in the metal–organic framework UiO-66

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