Issue 34, 2023

Selective CO2 hydrogenation over zeolite-based catalysts for targeted high-value products

Abstract

Catalytic conversion of CO2 to renewable fuels and green chemicals is a promising approach to utilize the large amount of CO2 generated from fossil fuels. The selectivity of targeted products is a critical parameter for effective CO2 conversion. However, the uncontrollable C–C coupling limits the selectivity of the desired products. This review focuses on recent advancements in CO2 hydrogenation over zeolite-based catalysts, with an emphasis on the selectivity of targeted products, such as methanol, olefins, and C5+ products. The role of zeolite properties, such as topology, acid sites, and metal–zeolite interactions, in determining product selectivity is comprehensively reviewed. Furthermore, recent progress in designing and modifying zeolite materials with enhanced CO2 conversion and targeted product selectivity is examined. The current technical challenges and perspectives for developing new zeolite-based catalysts for more efficient CO2 conversion are also discussed.

Graphical abstract: Selective CO2 hydrogenation over zeolite-based catalysts for targeted high-value products

Article information

Article type
Review Article
Submitted
28 may 2023
Accepted
07 avq 2023
First published
09 avq 2023

J. Mater. Chem. A, 2023,11, 17938-17960

Selective CO2 hydrogenation over zeolite-based catalysts for targeted high-value products

P. Yan, H. Peng, J. Vogrin, H. Rabiee and Z. Zhu, J. Mater. Chem. A, 2023, 11, 17938 DOI: 10.1039/D3TA03150K

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