Issue 19, 2021

A supramolecular dual-donor artificial light-harvesting system with efficient visible light-harvesting capacity

Abstract

The design and fabrication of highly efficient artificial light-harvesting systems (LHSs) are of great importance in supramolecular chemistry and materials science. Benefitting from the convenient construction process of supramolecular self-assembly, herein, a dual-donor artificial LHS was efficiently constructed through hierarchical self-assembly approaches involving metal–ligand coordination interactions, host–guest interactions and hydrophobic interactions. Notably, compared to the model single-donor artificial LHS with only one donor chromophore, the prepared dual-donor artificial LHS exhibited higher energy transfer efficiency and antenna effects. This research provides an efficient strategy for the construction of artificial LHSs with high energy transfer efficiency and antenna effects.

Graphical abstract: A supramolecular dual-donor artificial light-harvesting system with efficient visible light-harvesting capacity

Supplementary files

Article information

Article type
Research Article
Submitted
21 may 2021
Accepted
14 iyl 2021
First published
27 iyl 2021

Org. Chem. Front., 2021,8, 5250-5257

A supramolecular dual-donor artificial light-harvesting system with efficient visible light-harvesting capacity

Y. Hu, P. Jia, C. Zhang, X. Xu, Y. Niu, X. Zhao, Q. Xu, L. Xu and H. Yang, Org. Chem. Front., 2021, 8, 5250 DOI: 10.1039/D1QO00771H

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