Gradient static-strain stimulation in a microfluidic chip for 3D cellular alignment

Hsin-Yi Hsieh, Gulden Camci-Unal, Tsu-Wei Huang, Ronglih Liao, Tsung-Ju Chen, Arghya Paul, Fan-Gang Tseng and Ali Khademhosseini

Lab Chip, 2014, 14, 482
DOI: 10.1039/C3LC50884F

Transforming non-adhesive hydrogels to reversible tough adhesives via mixed-solvent-induced phase separation

Wei Cui, Ruijie Zhu, Yong Zheng, Qifeng Mu, Menghan Pi, Qiang Chen and Rong Ran

J. Mater. Chem. A, 2021, 9, 9706
DOI: 10.1039/D1TA00433F

Single network double cross-linker (SNDCL) hydrogels with excellent stretchability, self-recovery, adhesion strength, and conductivity for human motion monitoring

Zhenghao Li, Xiangxin Meng, Wenlong Xu, Shiqiang Zhang, Jiahui Ouyang, Zhuo Zhang, Yihan Liu, Yuzhong Niu, Songmei Ma, Zhongxin Xue, Aixin Song, Shaohua Zhang and Chunguang Ren

Soft Matter, 2020, 16, 7323
DOI: 10.1039/D0SM00375A

Strong, tough and mechanically self-recoverable poly(vinyl alcohol)/alginate dual-physical double-network hydrogels with large cross-link density contrast

Xuefeng Li, Mengmeng Shu, Han Li, Xiang Gao, Shijun Long, Tao Hu and Chonggang Wu

RSC Adv., 2018, 8, 16674
DOI: 10.1039/C8RA01302K

Synthetic self-assembled homogeneous network hydrogels with high mechanical and recoverable properties for tissue replacement

Yan-Jun Liu, Lian-Hua Fu, Shan Liu, Ling-Yan Meng, Ya-Yu Li and Ming-Guo Ma

J. Mater. Chem. B, 2016, 4, 4847
DOI: 10.1039/C6TB01249C

Fundamentals of double network hydrogels

Qiang Chen, Hong Chen, Lin Zhu and Jie Zheng

J. Mater. Chem. B, 2015, 3, 3654
DOI: 10.1039/C5TB00123D

Double network hydrogels prepared from pH-responsive doubly crosslinked microgels

Thomas Lane, Julianne L. Holloway, Amir H. Milani, Jennifer M. Saunders, Anthony J. Freemont and Brian R. Saunders

Soft Matter, 2013, 9, 7934
DOI: 10.1039/c3sm51356d

Polyacrylamide crosslinked by bis-vinylimidazolium bromide for high elastic and stable hydrogels

Caihong Wang, Xiaoqin Guan, Yongli Yuan, Yong Wu and Shuai Tan

RSC Adv., 2019, 9, 27640
DOI: 10.1039/C9RA05201A

Multiple hierarchical dynamic interactions enabled a robust, stretchable and room temperature self-healing elastomer

Jianfeng Fan, Xinqin Zhou and Yukun Chen

Polym. Chem., 2023, 14, 2117
DOI: 10.1039/D3PY00187C

The energy dissipation and Mullins effect of tough polymer/graphene oxide hybrid nanocomposite hydrogels

Ziqing Tang, Feng Chen, Qiang Chen, Lin Zhu, Xiaoqiang Yan, Hong Chen, Baiping Ren, Jia Yang, Gang Qin and Jie Zheng

Polym. Chem., 2017, 8, 4659
DOI: 10.1039/C7PY01068K

Mechanically strong triple network hydrogels based on hyaluronan and poly(N,N-dimethylacrylamide)

Burak Tavsanli, Volkan Can and Oguz Okay

Soft Matter, 2015, 11, 8517
DOI: 10.1039/C5SM01941A

Tough hybrid microgel-reinforced hydrogels dependent on the size and modulus of the microgels

Chun Li, Xiaohu Zhou, Lifei Zhu, Ziyao Xu, Peng Tan, Haifei Wang, Guokang Chen and Xuechang Zhou

Soft Matter, 2021, 17, 1566
DOI: 10.1039/D0SM01703E

Hydrogels toughened by biominerals providing energy-dissipative sacrificial bonds

Kazuki Fukao, Kazuki Tanaka, Ryuji Kiyama, Takayuki Nonoyama and Jian Ping Gong

J. Mater. Chem. B, 2020, 8, 5184
DOI: 10.1039/D0TB00833H

Highly stretchable cell-cultured hydrogel sheet

Kuniaki Nagamine, Yuina Abe, Hiroyuki Kai, Hirokazu Kaji and Matsuhiko Nishizawa

RSC Adv., 2015, 5, 66334
DOI: 10.1039/C5RA11059A

Simulational insights into the mechanical response of prestretched double network filled elastomers

Wenhui Wang, Zhiyu Zhang, Theodoros Davris, Jun Liu, Yangyang Gao, Liqun Zhang and Alexey V. Lyulin

Soft Matter, 2017, 13, 8597
DOI: 10.1039/C7SM01794D

Lipstick structure revealed by multimodal strain- and time-dependent rheology

Marie Gautier, Theany To, Anne-Sophie Botte, Jules Dupire, Tanguy Rouxel and Franck Artzner

Soft Matter, 2026, 22, 1739
DOI: 10.1039/D5SM01032B

Tough nanocomposite double network hydrogels reinforced with clay nanorods through covalent bonding and reversible chain adsorption

Guorong Gao, Gaolai Du, Yajun Cheng and Jun Fu

J. Mater. Chem. B, 2014, 2, 1539
DOI: 10.1039/c3tb21554g

Effects of chain flexibility on the properties of DNA hydrogels

Wei Pan, Hao Wen, Lin Niu, Cuicui Su, Chenyang Liu, Jiang Zhao, Chengde Mao and Dehai Liang

Soft Matter, 2016, 12, 5537
DOI: 10.1039/C6SM00283H

Quasi-unidirectional shrinkage of gels with well-oriented lipid bilayers upon uniaxial stretching

Tasuku Nakajima, Corentin Durand, Xu Feng Li, Md. Anamul Haque, Takayuki Kurokawa and Jian Ping Gong

Soft Matter, 2015, 11, 237
DOI: 10.1039/C4SM02113D

Effect of the constituent networks of double-network gels on their mechanical properties and energy dissipation process

Tasuku Nakajima, Takayuki Kurokawa, Hidemitsu Furukawa and Jian Ping Gong

Soft Matter, 2020, 16, 8618
DOI: 10.1039/D0SM01057J

Damage cross-effect and anisotropy in tough double network hydrogels revealed by biaxial stretching

Thanh-Tam Mai, Takahiro Matsuda, Tasuku Nakajima, Jian Ping Gong and Kenji Urayama

Soft Matter, 2019, 15, 3719
DOI: 10.1039/C9SM00409B

Multi-scale multi-mechanism design of tough hydrogels: building dissipation into stretchy networks

Xuanhe Zhao

Soft Matter, 2014, 10, 672
DOI: 10.1039/C3SM52272E

A phase diagram of neutral polyampholyte – from solution to tough hydrogel

Abu Bin Ihsan, Tao Lin Sun, Shinya Kuroda, Md. Anamul Haque, Takayuki Kurokawa, Tasuku Nakajima and Jian Ping Gong

J. Mater. Chem. B, 2013, 1, 4555
DOI: 10.1039/c3tb20790k

Highly robust hydrogels via a fast, simple and cytocompatible dual crosslinking-based process

Ana M. S. Costa and João F. Mano

Chem. Commun., 2015, 51, 15673
DOI: 10.1039/C5CC05564D

Nonlinear behavior of stochastic athermal fiber networks with elastic–plastic fibers

Syed N. Amjad, Nishan Parvez and Catalin R. Picu

Soft Matter, 2025, 21, 2882
DOI: 10.1039/D4SM01427H

Experimental study on crack repair materials for masonry ancient building based on skeleton effect

Jianwei Yue, Yaolin Li, Limin Zhao, Jiachang Chen, Qiang Deng, Zhixiang Shi and Zihao Guo

Journal of Building Engineering, 2024, 98, 111442
DOI: 10.1016/j.jobe.2024.111442

Kurt M. Schmoller and Andreas R. Bausch

Nature Mater, 2013, 12, 278
DOI: 10.1038/nmat3603

Anisotropic Swelling in Fiber-Reinforced Hydrogels: An Incremental Finite Element Method and Its Applications in Design of Bilayer Structures

Yin Liu, Hongwu Zhang, Jianhua Wang and Yonggang Zheng

Int. J. Appl. Mechanics, 2016, 08, 1640003
DOI: 10.1142/S1758825116400032

Distinctive Characteristics of Internal Fracture in Tough Double Network Hydrogels Revealed by Various Modes of Stretching

Thanh-Tam Mai, Takahiro Matsuda, Tasuku Nakajima, Jian Ping Gong and Kenji Urayama

Macromolecules, 2018, 51, 5245
DOI: 10.1021/acs.macromol.8b01033

Microscopic insights into the failure of elastic double networks

Justin Tauber, Simone Dussi and Jasper van der Gucht

Phys. Rev. Materials, 2020, 4
DOI: 10.1103/PhysRevMaterials.4.063603

Multi-layered PLLA-nanosheets loaded with FGF-2 induce robust bone regeneration with controlled release in critical-sized mouse femoral defects

Yasutaka Murahashi, Fumiko Yano, Hideki Nakamoto, Yuji Maenohara, Kousuke Iba, Toshihiko Yamashita, Sakae Tanaka, Kazuhiko Ishihara, Yosuke Okamura, Toru Moro and Taku Saito

Acta Biomaterialia, 2019, 85, 172
DOI: 10.1016/j.actbio.2018.12.031

A mesoscopic theory to describe the flexibility regulation in F-actin networks: An approach of phase transitions with nonlinear elasticity

Horacio Lopez-Menendez

Journal of the Mechanical Behavior of Biomedical Materials, 2020, 101, 103432
DOI: 10.1016/j.jmbbm.2019.103432

The Fracture of Highly Deformable Soft Materials: A Tale of Two Length Scales

Rong Long, Chung-Yuen Hui, Jian Ping Gong and Eran Bouchbinder

Annu. Rev. Condens. Matter Phys., 2021, 12, 71
DOI: 10.1146/annurev-conmatphys-042020-023937

The stress field near the tip of a plane stress crack in a gel consisting of chemical and physical cross-links

Jingyi Guo, Chung-Yuen Hui, Mincong Liu and Alan T. Zehnder

Proc. R. Soc. A., 2019, 475, 20180863
DOI: 10.1098/rspa.2018.0863

A Solvent‐Exchange Strategy to Regulate Noncovalent Interactions for Strong and Antiswelling Hydrogels

Liju Xu, Shan Gao, Qirui Guo, Chen Wang, Yan Qiao and Dong Qiu

Advanced Materials, 2020, 32
DOI: 10.1002/adma.202004579

Crack Tip Field of a Double-Network Gel: Visualization of Covalent Bond Scission through Mechanoradical Polymerization

Takahiro Matsuda, Runa Kawakami, Tasuku Nakajima and Jian Ping Gong

Macromolecules, 2020, 53, 8787
DOI: 10.1021/acs.macromol.0c01485

Improving the strength and toughness of macroscale double networks by exploiting Poisson’s ratio mismatch

Tsuyoshi Okumura, Riku Takahashi, Katsumi Hagita, Daniel R. King and Jian Ping Gong

Sci Rep, 2021, 11
DOI: 10.1038/s41598-021-92773-0

Advances and challenges in conductive hydrogels: From properties to applications

Can Zhou, Tingting Wu, Xinmin Xie, Guoxi Song, Xintao Ma, Qiyu Mu, Zixu Huang, Xiguang Liu, Changmei Sun and Wenlong Xu

European Polymer Journal, 2022, 177, 111454
DOI: 10.1016/j.eurpolymj.2022.111454

Solvent and Ca2+ triggered robust and fast stress generation by ultrathin triple-network hydrogels

Songmiao Liang, Jian Hu, Zi Liang Wu, Takayuki Kurokawa and Jian Ping Gong

Extreme Mechanics Letters, 2014, 1, 17
DOI: 10.1016/j.eml.2014.10.002

Fabrication of Tough Hydrogel Composites from Photoresponsive Polymers to Show Double-Network Effect

Zhen Tao, Hailong Fan, Junchao Huang, Taolin Sun, Takayuki Kurokawa and Jian Ping Gong

ACS Appl. Mater. Interfaces, 2019, 11, 37139
DOI: 10.1021/acsami.9b13746

Highly selective CO2 permeable double-network ionogel membrane containing 1-ethyl-3-methylimidazolium dicyanamide

Shengnan He, Eiji Kamio, Atsushi Matsuoka, Keizo Nakagawa, Tomohisa Yoshioka and Hideto Matsuyama

Journal of Membrane Science, 2024, 711, 123200
DOI: 10.1016/j.memsci.2024.123200

Fabrication of Tough Double-Network Hydrogels from Highly Cross-Linked Brittle Neutral Networks Using Alkaline Hydrolysis

S. Shams Es-haghi and R. A. Weiss

Gels, 2023, 10, 29
DOI: 10.3390/gels10010029

Improvement of Mechanical Strength and Fatigue Resistance of Double Network Hydrogels by Ionic Coordination Interactions

Qiang Chen, Xiaoqiang Yan, Lin Zhu, Hong Chen, Bing Jiang, Dandan Wei, Lina Huang, Jia Yang, Baozhong Liu and Jie Zheng

Chem. Mater., 2016, 28, 5710
DOI: 10.1021/acs.chemmater.6b01920

A theory to describe emergent properties of composite F-actin and vimentin networks

Horacio Lopez-Menendez and Libardo Gonzalez-Torres

Journal of the Mechanics and Physics of Solids, 2019, 127, 208
DOI: 10.1016/j.jmps.2019.03.017

Finite strain theory of a Mode III crack in a rate dependent gel consisting of chemical and physical cross-links

Chung Yuen Hui, Jingyi Guo, Mincong Liu and Alan Zehnder

Int J Fract, 2019, 215, 77
DOI: 10.1007/s10704-018-00335-9

An ultra-stretchable glycerol-ionic hybrid hydrogel with reversible gelid adhesion

Yonggan Yan, Jun Huang, Xiaoyong Qiu, Xin Cui, Shulei Xu, Xunwei Wu, Peng Yao and Chuanzhen Huang

Journal of Colloid and Interface Science, 2021, 582, 187
DOI: 10.1016/j.jcis.2020.08.008

Inverse mechanical-swelling coupling of a highly deformed double-network gel

Chika Imaoka, Tasuku Nakajima, Tsutomu Indei, Masaya Iwata, Wei Hong, Alba Marcellan and Jian Ping Gong

Sci. Adv., 2023, 9
DOI: 10.1126/sciadv.abp8351

Synthesis and characterization of robust double-networks based on end-linked, pH-responsive first networks

Elina N. Kitiri, Maria Rikkou-Kalourkoti, Manolia Sophocleous and Costas S. Patrickios

European Polymer Journal, 2015, 69, 573
DOI: 10.1016/j.eurpolymj.2015.02.002

Large deformation near a crack tip in a fiber-reinforced neo-Hookean sheet with discrete and continuous distributions of fiber orientations

Luca Di Stasio, Yin Liu and Brian Moran

Theoretical and Applied Fracture Mechanics, 2021, 114, 103020
DOI: 10.1016/j.tafmec.2021.103020

Fracture mechanics of blood clots: Measurements of toughness and critical length scales

Shiyu Liu, Guangyu Bao, Zhenwei Ma, Christian J. Kastrup and Jianyu Li

Extreme Mechanics Letters, 2021, 48, 101444
DOI: 10.1016/j.eml.2021.101444

Azo-Crosslinked Double-Network Hydrogels Enabling Highly Efficient Mechanoradical Generation

Zhi Jian Wang, Julong Jiang, Qifeng Mu, Satoshi Maeda, Tasuku Nakajima and Jian Ping Gong

J. Am. Chem. Soc., 2022, 144, 3154
DOI: 10.1021/jacs.1c12539

Strikingly improved toughness of nonpolar rubber by incorporating sacrificial network at small fraction

Xuhui Zhang, Zhenghai Tang, Jing Huang, Tengfei Lin and Baochun Guo

J Polym Sci B Polym Phys, 2016, 54, 781
DOI: 10.1002/polb.23980

Topoarchitected Polymer Network Hydrogels with High Toughness and Anisotropic Properties

Xiao Liu, Xuyan Yang, Jingping Wu, Hongfei He, Xueqi Zhao, Keke Qiao, Yong Zheng and Jian Hu

Macromolecules, 2025, 58, 3993
DOI: 10.1021/acs.macromol.5c00043

Fundamental toughening landscape in soft–hard composites: Insights from a minimal framework

Fucheng Tian, Katsuhiko Sato, Yong Zheng, Feixue Lu and Jian Ping Gong

Proc. Natl. Acad. Sci. U.S.A., 2025, 122
DOI: 10.1073/pnas.2506071122

Bioelectronics hydrogels for implantable cardiac and brain disease medical treatment application

Yanfang Meng, Lin Xu and Guanggui Cheng

International Journal of Biological Macromolecules, 2025, 299, 139945
DOI: 10.1016/j.ijbiomac.2025.139945

Scaling dynamics of globule-to-coil phase transition in double-network hydrogel with ultra-high stretchable strength

Haibao Lu, Ziyu Xing, Mokarram Hossain and Jinsong Leng

Smart Mater. Struct., 2020, 29, 085050
DOI: 10.1088/1361-665X/ab9e0c

Nonionic Double and Triple Network Hydrogels of High Mechanical Strength

Aslihan Argun, Volkan Can, Ugur Altun and Oguz Okay

Macromolecules, 2014, 47, 6430
DOI: 10.1021/ma5014176

Generalization of the sacrificial bond principle for gel and elastomer toughening

Tasuku Nakajima

Polym J, 2017, 49, 477
DOI: 10.1038/pj.2017.12

A Dual-Responsive, Freezing-Tolerant Hydrogel Sensor and Related Thermal- and Strain-Sensitive Mechanisms

Yonggan Yan, Luxing Wei, Xiaoyong Qiu, Jinlong Shao, Hanlian Liu, Xin Cui, Jun Huang, Lei Xie, Zhenfeng Hu and Chuanzhen Huang

ACS Appl. Polym. Mater., 2021, 3, 1479
DOI: 10.1021/acsapm.0c01346

Effect of Relative Strength of Two Networks on the Internal Fracture Process of Double Network Hydrogels As Revealed by in Situ Small-Angle X-ray Scattering

Kazuki Fukao, Tasuku Nakajima, Takayuki Nonoyama, Takayuki Kurokawa, Takahiko Kawai and Jian Ping Gong

Macromolecules, 2020, 53, 1154
DOI: 10.1021/acs.macromol.9b02562

Synthesis and Fracture Process Analysis of Double Network Hydrogels with a Well-Defined First Network

Tasuku Nakajima, Yuki Fukuda, Takayuki Kurokawa, Takamasa Sakai, Ung-il Chung and Jian Ping Gong

ACS Macro Lett., 2013, 2, 518
DOI: 10.1021/mz4002047

Tough Double-Network Gels and Elastomers from the Nonprestretched First Network

Tasuku Nakajima, Yuhei Ozaki, Ryo Namba, Kumi Ota, Yuki Maida, Takahiro Matsuda, Takayuki Kurokawa and Jian Ping Gong

ACS Macro Lett., 2019, 8, 1407
DOI: 10.1021/acsmacrolett.9b00679

Understanding complex dynamics of interfacial reconstruction in polyampholyte hydrogels undergoing mechano-chemo-electrotaxis coupling

Ziyu Xing, Haibao Lu, Ansu Sun, Yong Qing Fu, Muhammad Wakil Shahzad and Ben Bin Xu

J. Phys. D: Appl. Phys., 2021, 54, 085301
DOI: 10.1088/1361-6463/abc649

A Novel Design Strategy for Fully Physically Linked Double Network Hydrogels with Tough, Fatigue Resistant, and Self‐Healing Properties

Qiang Chen, Lin Zhu, Hong Chen, Hongli Yan, Lina Huang, Jia Yang and Jie Zheng

Adv Funct Materials, 2015, 25, 1598
DOI: 10.1002/adfm.201404357

Network from Dihydrocoumarin via Solvent-Free Metal-Mediated Pathway: A Potential Structure for Substantial Toughness Improvement of Epoxidized Plant Oil Materials

Cong Li, Jonggeun Sung and Xiuzhi Susan Sun

ACS Sustainable Chem. Eng., 2016, 4, 1231
DOI: 10.1021/acssuschemeng.5b01283

Characterization of stress softening and self-healing in a double network hydrogel

İsmail Doğan Külcü

Results in Physics, 2019, 12, 1826
DOI: 10.1016/j.rinp.2019.01.078

Revealing novel insights into the toughening mechanism of double network hydrogels via uniaxial tensile tests

Jiapeng You and Zishun Liu

Journal of the Mechanics and Physics of Solids, 2024, 190, 105710
DOI: 10.1016/j.jmps.2024.105710

Nanophase Separation in Immiscible Double Network Elastomers Induces Synergetic Strengthening, Toughening, and Fatigue Resistance

Yong Zheng, Ryuji Kiyama, Takahiro Matsuda, Kunpeng Cui, Xueyu Li, Wei Cui, Yunzhou Guo, Tasuku Nakajima, Takayuki Kurokawa and Jian Ping Gong

Chem. Mater., 2021, 33, 3321
DOI: 10.1021/acs.chemmater.1c00512

Rapid room-temperature preparation and hydrovoltaic application of biohydrogel

MingQiu HONG, GuoPing REN, QiChang HU, Jie YE and ShunGui ZHOU

Sci. Sin.-Tech., 2025, 55, 104
DOI: 10.1360/SST-2024-0122

Revisiting the Origins of the Fracture Energy of Tough Double-Network Hydrogels with Quantitative Mechanochemical Characterization of the Damage Zone

Takahiro Matsuda, Runa Kawakami, Tasuku Nakajima, Yukiko Hane and Jian Ping Gong

Macromolecules, 2021, 54, 10331
DOI: 10.1021/acs.macromol.1c01214

Mechanics of Physically Cross-Linked Hydrogels: Experiments and Theoretical Modeling

Mohit Goswami, Agniva Dutta, Rishi Kulshreshtha, Gleb Vasilyev, Eyal Zussman and Konstantin Volokh

Macromolecules, 2025, 58, 4478
DOI: 10.1021/acs.macromol.5c00486

Toughening hydrogels through force-triggered chemical reactions that lengthen polymer strands

Zi Wang, Xujun Zheng, Tetsu Ouchi, Tatiana B. Kouznetsova, Haley K. Beech, Sarah Av-Ron, Takahiro Matsuda, Brandon H. Bowser, Shu Wang, Jeremiah A. Johnson, Julia A. Kalow, Bradley D. Olsen, Jian Ping Gong, Michael Rubinstein and Stephen L. Craig

Science, 2021, 374, 193
DOI: 10.1126/science.abg2689

Facile Fabrication of Tough, Low-Temperature Flexible Conductive Hydrogels via Solvent Competition-Induced Crystallization

Dongchao Ji, Xiaoman Fei, Guangpeng Wang, Xiaolei Wang, Lei Yang, Zhuochao Wang, Zhibo Zhang, Wenxin Cao, Jiecai Han and Jiaqi Zhu

ACS Appl. Electron. Mater., 2025, 7, 7872
DOI: 10.1021/acsaelm.5c01240

Rubber-reinforced rubbers toward the combination of high reinforcement and low energy loss

Shifeng Fang, Fanzhu Li, Jun Liu, Liqun Zhang, Dong Wang, Bin Liu, Siwu Wu, Zhenghai Tang and Baochun Guo

Nano Energy, 2021, 83, 105822
DOI: 10.1016/j.nanoen.2021.105822

Toughening Elastomers with Sacrificial Bonds and Watching Them Break

Etienne Ducrot, Yulan Chen, Markus Bulters, Rint P. Sijbesma and Costantino Creton

Science, 2014, 344, 186
DOI: 10.1126/science.1248494

Characterization of the deformation and fracture of tough double-network hydrogels

Sitao Wang, Eric Euchler, Konrad Schneider and Sven Wießner

Polymer, 2025, 340, 129190
DOI: 10.1016/j.polymer.2025.129190

A Constitutive Model for Alginate-Based Double Network Hydrogels Cross-Linked by Mono-, Di-, and Trivalent Cations

İsmail Doğan Külcü

Gels, 2020, 7, 3
DOI: 10.3390/gels7010003

Innovative approaches in bioadhesive design: A comprehensive review of crosslinking methods and mechanical performance

Asef Raj, Sabrina Sharmin, Safrin Jannat, Saika Ahmed and Abu Bin Ihsan

Biomaterials Advances, 2025, 173, 214287
DOI: 10.1016/j.bioadv.2025.214287

Fatigue of double-network hydrogels

Wenlei Zhang, Xiao Liu, Jikun Wang, Jingda Tang, Jian Hu, Tongqing Lu and Zhigang Suo

Engineering Fracture Mechanics, 2018, 187, 74
DOI: 10.1016/j.engfracmech.2017.10.018

A multi-functional reversible hydrogel adhesive

Yonggan Yan, Shulei Xu, Huanxi Liu, Xin Cui, Jinlong Shao, Peng Yao, Jun Huang, Xiaoyong Qiu and Chuanzhen Huang

Colloids and Surfaces A: Physicochemical and Engineering Aspects, 2020, 593, 124622
DOI: 10.1016/j.colsurfa.2020.124622

Stretchy and disordered: Toward understanding fracture in soft network materials via mesoscopic computer simulations

Justin Tauber, Jasper van der Gucht and Simone Dussi

The Journal of Chemical Physics, 2022, 156
DOI: 10.1063/5.0081316

Constitutive modeling of bond breaking and healing kinetics of physical Polyampholyte (PA) gel

Sairam Pamulaparthi Venkata, Kunpeng Cui, Jingyi Guo, Alan T. Zehnder, Jian Ping Gong and Chung-Yuen Hui

Extreme Mechanics Letters, 2021, 43, 101184
DOI: 10.1016/j.eml.2021.101184

Preparation and fracture process of high strength hyaluronic acid hydrogels cross-linked by ethylene glycol diglycidyl ether

Burak Tavsanli and Oguz Okay

Reactive and Functional Polymers, 2016, 109, 42
DOI: 10.1016/j.reactfunctpolym.2016.10.001

A theory of finite tensile deformation of double‐network hydrogels

Siamak Shams Es‐haghi and Robert A. Weiss

Journal of Polymer Science, 2022, 60, 2476
DOI: 10.1002/pol.20220140

A damage model of characterizing the internal damage evolution for DN hydrogel using Multi-Particle Tracking (MPT) method

Chong Wang, Yetong Jia, Jiapeng You, Jincheng Lei and Zishun Liu

Mechanics of Materials, 2025, 206, 105360
DOI: 10.1016/j.mechmat.2025.105360

Ultra-high strength poly(N-(2-hydroxyethyl)acrylamide)/chitosan hydrogel with “repelling and killing” bacteria property

Jing Zhang, Lingdong Chen, Biao Shen, Liqun Chen and Jie Feng

Carbohydrate Polymers, 2019, 225, 115160
DOI: 10.1016/j.carbpol.2019.115160

Simultaneous One‐Pot Interpenetrating Network Formation to Expand 3D Processing Capabilities

Abhishek P. Dhand, Matthew D. Davidson, Jonathan H. Galarraga, Taimoor H. Qazi, Ryan C. Locke, Robert L. Mauck and Jason A. Burdick

Advanced Materials, 2022, 34
DOI: 10.1002/adma.202202261

Fatigue of hydrogels

Ruobing Bai, Jiawei Yang and Zhigang Suo

European Journal of Mechanics - A/Solids, 2019, 74, 337
DOI: 10.1016/j.euromechsol.2018.12.001

A compact anisotropic model for the mechanical response of double network hydrogels

Domenico De Tommasi, Francesco Trentadue and Gennaro Vitucci

International Journal of Engineering Science, 2026, 220, 104437
DOI: 10.1016/j.ijengsci.2025.104437

Fracture of the Physically Cross-Linked First Network in Hybrid Double Network Hydrogels

Qiang Chen, Lin Zhu, Lina Huang, Hong Chen, Kun Xu, Yin Tan, Pixin Wang and Jie Zheng

Macromolecules, 2014, 47, 2140
DOI: 10.1021/ma402542r

Influence of the Degree of Swelling on the Stiffness and Toughness of Microgel‐Reinforced Hydrogels

Michael Kessler, Tianyu Yuan, John M. Kolinski and Esther Amstad

Macromol. Rapid Commun., 2023, 44
DOI: 10.1002/marc.202200864

Bioinspired Ion-Mediated Repair Strategy for Irreversibly Covalently Cross-Linked Double-Network Hydrogels

Xiaoyu He, Qifeng Mu, Huanwei Shen, Min Li, Xiayue Yang, Menghan Pi, Longyu Hu, Wei Cui and Rong Ran

Macromolecules, 2026, 59, 2742
DOI: 10.1021/acs.macromol.5c02758

Sharing the Load: Stress Redistribution Governs Fracture of Polymer Double Networks

Justin Tauber, Lorenzo Rovigatti, Simone Dussi and Jasper van der Gucht

Macromolecules, 2021, 54, 8563
DOI: 10.1021/acs.macromol.1c01275

Nanostructure Evolution during Relaxation from a Large Step Strain in a Supramolecular Copolymer-Based Hydrogel: A SANS Investigation

Clinton G. Wiener, Chao Wang, Yun Liu, R. A. Weiss and Bryan D. Vogt

Macromolecules, 2017, 50, 1672
DOI: 10.1021/acs.macromol.6b02680

A Micromechanically Based Constitutive Model for the Inelastic and Swelling Behaviors in Double Network Hydrogels

Yin Liu, Hongwu Zhang and Yonggang Zheng

Journal of Applied Mechanics, 2016, 83
DOI: 10.1115/1.4031897

Fracture Process Analysis and Deformation-Induced Toughening of Double-Network Gels

Tasuku Nakajima

J. Soc. Rheol., Jpn, 2022, 50, 359
DOI: 10.1678/rheology.50.359

Extremely strong and tough hydrogels as prospective candidates for tissue repair – A review

Ana M.S. Costa and João F. Mano

European Polymer Journal, 2015, 72, 344
DOI: 10.1016/j.eurpolymj.2015.07.053

Mechanical response of HEMA gel under cyclic deformation: Viscoplasticity and swelling-induced recovery

A.D. Drozdov, C.-G. Sanporean and J. de C. Christiansen

International Journal of Solids and Structures, 2015, 52, 220
DOI: 10.1016/j.ijsolstr.2014.10.009

Internal Damage Evolution in Double-Network Hydrogels Studied by Microelectrode Technique

Honglei Guo, Wei Hong, Takayuki Kurokawa, Takahiro Matsuda, Zi Liang Wu, Tasuku Nakajima, Masakazu Takahata, Taolin Sun, Ping Rao and Jian Ping Gong

Macromolecules, 2019, 52, 7114
DOI: 10.1021/acs.macromol.9b01308

Anisotropic stress-softening effect on fast dynamic crack in filler-reinforced elastomers

Thanh-Tam Mai, Kenichiro Okuno, Katsuhiko Tsunoda and Kenji Urayama

Mechanics of Materials, 2021, 155, 103786
DOI: 10.1016/j.mechmat.2021.103786

“Nonswellable” Hydrogel Without Mechanical Hysteresis

Hiroyuki Kamata, Yuki Akagi, Yuko Kayasuga-Kariya, Ung-il Chung and Takamasa Sakai

Science, 2014, 343, 873
DOI: 10.1126/science.1247811

Fracture and adhesion of soft materials: a review

Costantino Creton and Matteo Ciccotti

Rep. Prog. Phys., 2016, 79, 046601
DOI: 10.1088/0034-4885/79/4/046601

Chitin-Based Double-Network Hydrogel as Potential Superficial Soft-Tissue-Repairing Materials

Junchao Huang, Martin Frauenlob, Yuki Shibata, Lei Wang, Tasuku Nakajima, Takayuki Nonoyama, Masumi Tsuda, Shinya Tanaka, Takayuki Kurokawa and Jian Ping Gong

Biomacromolecules, 2020, 21, 4220
DOI: 10.1021/acs.biomac.0c01003

Deformation Behavior of Fiber-Reinforced Hydrogel Structures

Yu Zhou, Jianying Hu and Zishun Liu

Int. J. Str. Stab. Dyn., 2019, 19, 1950032
DOI: 10.1142/S0219455419500329

Dual Physically Cross-Linked κ-Carrageenan-Based Double Network Hydrogels with Superior Self-Healing Performance for Biomedical Application

Yi Deng, Min Huang, Dan Sun, Yi Hou, Yubao Li, Taosheng Dong, Xiaohong Wang, Li Zhang and Weizhong Yang

ACS Appl. Mater. Interfaces, 2018, 10, 37544
DOI: 10.1021/acsami.8b15385

Constitutive modeling for polymer hydrogels: A new perspective and applications to anisotropic hydrogels in free swelling

Yin Liu, Hongwu Zhang, Jiayong Zhang and Yonggang Zheng

European Journal of Mechanics - A/Solids, 2015, 54, 171
DOI: 10.1016/j.euromechsol.2015.07.001

Macroscale double networks: highly dissipative soft composites

Daniel R. King

Polym J, 2022, 54, 943
DOI: 10.1038/s41428-022-00646-8

Extremely Stretchable Vitrimers

Zhenyu Lyu and Tongfei Wu

Macromol. Rapid Commun., 2020, 41
DOI: 10.1002/marc.202000265

Predicting fracture toughness of double network hydrogel via monotonic loading test

Jiapeng You and Zishun Liu

Polymer, 2026, 345, 129573
DOI: 10.1016/j.polymer.2026.129573

Simultaneous Enhancement of Stiffness and Toughness in Hybrid Double-Network Hydrogels via the First, Physically Linked Network

Qiang Chen, Dandan Wei, Hong Chen, Lin Zhu, Caicai Jiao, Ge Liu, Lina Huang, Jia Yang, Libo Wang and Jie Zheng

Macromolecules, 2015, 48, 8003
DOI: 10.1021/acs.macromol.5b01938

One‐Pot Fabrication of a Novel Agar‐Polyacrylamide/Graphene Oxide Nanocomposite Double Network Hydrogel with High Mechanical Properties

Pang Zhu, Meng Hu, Yonghong Deng and Chaoyang Wang

Adv Eng Mater, 2016, 18, 1799
DOI: 10.1002/adem.201600272

Yielding Criteria of Double Network Hydrogels

Takahiro Matsuda, Tasuku Nakajima, Yuki Fukuda, Wei Hong, Takamasa Sakai, Takayuki Kurokawa, Ung-il Chung and Jian Ping Gong

Macromolecules, 2016, 49, 1865
DOI: 10.1021/acs.macromol.5b02592

Rapid self-strengthening in double-network hydrogels triggered by bond scission

Zhi Jian Wang, Wei Li, Xueyu Li, Tasuku Nakajima, Michael Rubinstein and Jian Ping Gong

Nat. Mater., 2025, 24, 607
DOI: 10.1038/s41563-025-02137-6

Comparison of Mullins Effect Anisotropy of the Elastomers Reinforced by Carbon-Black and Silica Filler

Thanh-Tam Mai, Yuga Taniguchi, Katsuhiko Tsunoda and Kenji Urayama

J. Soc. Rheol., Jpn, 2023, 51, 33
DOI: 10.1678/rheology.51.33

A network alteration theory of rubbery polymers for exploring the damage and mechanochemistry

Ziyu Xing

International Journal of Engineering Science, 2025, 216, 104359
DOI: 10.1016/j.ijengsci.2025.104359

A combined numerical and theoretical study on the strengthening and toughening mechanisms of double network hydrogels

Bo Gong, Ji Lin, Yu Xie and Jin Qian

International Journal of Smart and Nano Materials, 2025, 16, 284
DOI: 10.1080/19475411.2025.2476130

Structure of Tough Multiple Network Elastomers by Small Angle Neutron Scattering

Etienne Ducrot, Helene Montes and Costantino Creton

Macromolecules, 2015, 48, 7945
DOI: 10.1021/acs.macromol.5b01979

Morphological and mechanical properties of tannic acid/PAAm semi-IPN hydrogels for cell adhesion

Xinyu Hu, Yongmei Wang, Liangliang Zhang and Man Xu

Polymer Testing, 2017, 61, 314
DOI: 10.1016/j.polymertesting.2017.05.034

Construction of polydopamine reduced graphene oxide/sodium carboxymethyl cellulose/polyacrylamide double network conductive hydrogel with high stretchable, pH-sensitive and strain-sensing properties

Huixian Yin, Shuo Li, Hanlin Xie, Yihao Wu, Xinquan Zou, Yicheng Huang and Jikui Wang

Colloids and Surfaces A: Physicochemical and Engineering Aspects, 2022, 642, 128428
DOI: 10.1016/j.colsurfa.2022.128428

Flexible and recoverable ion-conductive hydrogels with cross-linked triple network for highly sensitive wearable Motion-monitoring sensors

Weidi He, Feng Xu, Shengjun Lu, Yufei Zhang and Haosen Fan

Next Materials, 2023, 1, 100027
DOI: 10.1016/j.nxmate.2023.100027

Toughening epoxy resin by constructing π-π interaction between a tung oil-based modifier and epoxy

Laihui Xiao, Shuai Li, Yigang Wang, Wenbin Li, Jie Chen, Jinrui Huang and Xiaoan Nie

Industrial Crops and Products, 2021, 170, 113723
DOI: 10.1016/j.indcrop.2021.113723

Mechanics of elastomeric molecular composites

Pierre Millereau, Etienne Ducrot, Jess M. Clough, Meredith E. Wiseman, Hugh R. Brown, Rint P. Sijbesma and Costantino Creton

Proc. Natl. Acad. Sci. U.S.A., 2018, 115, 9110
DOI: 10.1073/pnas.1807750115

Cyclic tensile machine with wide speed range for in situ neutron/X-ray scattering study on elastomers

Nan Tian, Tingting Wang, Xiaoqing Tu, Yue Shui, Jianzhu Ju, Guangai Sun and Dong Liu

Review of Scientific Instruments, 2020, 91
DOI: 10.1063/1.5128047

Fabrication of a Double-Network Hydrogel Based on Carboxymethylated Curdlan/Polyacrylamide with Highly Mechanical Performance for Cartilage Repair

Pengguang Wang, Min Wu, Ruiqi Li, Zhixiang Cai and Hongbin Zhang

ACS Appl. Polym. Mater., 2021, 3, 5857
DOI: 10.1021/acsapm.1c01094

Modeling strategy for dynamic-modal mechanophore in double-network hydrogel composites with self-growing and tailorable mechanical strength

Haibao Lu, Ziyu Xing, Mokarram Hossain and Yong-Qing Fu

Composites Part B: Engineering, 2019, 179, 107528
DOI: 10.1016/j.compositesb.2019.107528

Polyacrylamide/sodium alginate photochromic hydrogels with enhanced toughness and fast response for optical display and rewritable information record

Xiangyong Wu, Xian Deng, Ying Song, Zhenxiao Zhang, Hao Su, Ying Han, Yihui Shen, Sitong Liu, Keying Sun, Hongyan Yao and Shaowei Guan

Dyes and Pigments, 2023, 210, 111009
DOI: 10.1016/j.dyepig.2022.111009

High-strength and tough composite hydrogels reinforced by the synergistic effect of nano-doping and triple-network structures

Jing-Hui Wang, Ya-Nan Xue, Yan-Qin Wang, Mei-Wen An, Yi-Xian Qin and Wei-Yi Chen

European Polymer Journal, 2021, 142, 110122
DOI: 10.1016/j.eurpolymj.2020.110122

Pre-yielding and necking process of double network hydrogels revealed by sample geometry effects

Masahiro Yoshida, Ryuji Kiyama, Ye Zhang, Daniel R. King, Takayuki Kurokawa and Jian Ping Gong

Extreme Mechanics Letters, 2024, 69, 102163
DOI: 10.1016/j.eml.2024.102163

Lignin-incorporated PVA/chitosan hydrogels with highly enhanced toughness and rigidity through a non-covalent crosslinking strategy

Yihui Gu, Haoyu Wang, Yufeng Yuan, Chaofeng Zhang, Wenjuan Wu, Wangxia Wang, M. Mostafizur Rahman, Bo Jiang and Yongcan Jin

Chemical Engineering Journal, 2026, 531, 173970
DOI: 10.1016/j.cej.2026.173970

Graphene Oxide/Polyacrylamide/Aluminum Ion Cross‐Linked Carboxymethyl Hemicellulose Nanocomposite Hydrogels with Very Tough and Elastic Properties

Weiqing Kong, Danyang Huang, Guibin Xu, Junli Ren, Chuanfu Liu, Lihong Zhao and Runcang Sun

Chemistry An Asian Journal, 2016, 11, 1697
DOI: 10.1002/asia.201600138

Fmoc-phenylalanine as a building block for hybrid double network hydrogels with enhanced mechanical properties, self-recovery, and shape memory capability

Jiseon Kang and Seok Il Yun

Polymer, 2022, 255, 125145
DOI: 10.1016/j.polymer.2022.125145

Toughening Hydrogels with Fibrillar Connected Double Networks

Yu‐Huang Fang, Chen Liang, Ville Liljeström, Zhong‐Peng Lv, Olli Ikkala and Hang Zhang

Advanced Materials, 2024, 36
DOI: 10.1002/adma.202402282

How Supertough Gels Break

Itamar Kolvin, John M. Kolinski, Jian Ping Gong and Jay Fineberg

Phys. Rev. Lett., 2018, 121
DOI: 10.1103/PhysRevLett.121.135501

Stretch-induced structural evolution of poly (vinyl alcohol) at different concentrations of boric acid: An in-situ synchrotron radiation small- and wide- angle X-ray scattering study

Ke Ye, Yahui Li, Wenwen Zhang, Qianlei Zhang, Wei Chen, Lingpu Meng, Daoliang Wang and Liangbin Li

Polymer Testing, 2019, 77, 105913
DOI: 10.1016/j.polymertesting.2019.105913

Preparation and Properties of Composite Double-Network Gel for Inhibiting Coal Spontaneous Combustion

Jianguo Wang, Zhenzhen Zhang, Wen Fu and Yifan Zhao

Molecules, 2024, 29, 3365
DOI: 10.3390/molecules29143365

Brittle–ductile transition of double network hydrogels: Mechanical balance of two networks as the key factor

Saika Ahmed, Tasuku Nakajima, Takayuki Kurokawa, Md. Anamul Haque and Jian Ping Gong

Polymer, 2014, 55, 914
DOI: 10.1016/j.polymer.2013.12.066

Swelling Effect on the Yielding, Elasticity, and Fracture of Double-Network Hydrogels with an Inhomogeneous First Network

Yong Zheng, Tasuku Nakajima, Wei Cui, Chung-Yuen Hui and Jian Ping Gong

Macromolecules, 2023, 56, 3962
DOI: 10.1021/acs.macromol.3c00354

Self-Regulating Hydrogel Actuators

Taehun Chung, Jaewon Choi, Takafumi Enomoto, Soyeon Park, Saehyun Kim and Youn Soo Kim

Chem. Rev., 2025, 125, 9053
DOI: 10.1021/acs.chemrev.5c00358

Strengthening Your Networks and Responding to Stress and Strain: What Humans in STEM Can Learn from Soft Matter and Biological Materials

Surita R. Bhatia and Jennifer L. Ross

Ind. Eng. Chem. Res., 2025, 64, 18077
DOI: 10.1021/acs.iecr.5c02000

Nonswelling Click-Cross-Linked Gelatin and PEG Hydrogels with Tunable Properties Using Pluronic Linkers

Vinh X. Truong, Kelly M. Tsang and John S. Forsythe

Biomacromolecules, 2017, 18, 757
DOI: 10.1021/acs.biomac.6b01601

Polysaccharide-Based Double-Network Hydrogels: Polysaccharide Effect, Strengthening Mechanisms, and Applications

Pengguang Wang, Qingyu Liao and Hongbin Zhang

Biomacromolecules, 2023, 24, 5479
DOI: 10.1021/acs.biomac.3c00765

A Chain Scission-Induced Anisotropic Damage Constitutive Model for Double Network Hydrogels

Jincheng Lei and Zishun Liu

Int. J. Appl. Mechanics, 2024, 16
DOI: 10.1142/S1758825124500765

Prolonged morphometric study of barnacles grown on soft substrata of hydrogels and elastomers

Nafees Ahmed, Takayuki Murosaki, Takayuki Kurokawa, Akira Kakugo, Shintaro Yashima, Yasuyuki Nogata and Jian Ping Gong

Biofouling, 2014, 30, 271
DOI: 10.1080/08927014.2013.863280

Anisotropic Growth of Hydroxyapatite in Stretched Double Network Hydrogel

Kazuki Fukao, Takayuki Nonoyama, Ryuji Kiyama, Kazuya Furusawa, Takayuki Kurokawa, Tasuku Nakajima and Jian Ping Gong

ACS Nano, 2017, 11, 12103
DOI: 10.1021/acsnano.7b04942

Swelling-strengthening hydrogels by embedding with deformable nanobarriers

Feng Wu, Yan Pang and Jinyao Liu

Nat Commun, 2020, 11
DOI: 10.1038/s41467-020-18308-9

Effect of the Second Network on First Network Rupture and the Origin of Energy Dissipation in Double Network Hydrogels

Zhi Jian Wang, Gumi Wei, Tasuku Nakajima and Jian Ping Gong

Macromolecules, 2025, 58, 4835
DOI: 10.1021/acs.macromol.5c00331

Yielding of Double-Network Hydrogels with Systematically Controlled Tetra-PEG First Networks

Takahiro Matsuda, Naohiro Kashimura, Takamasa Sakai, Tasuku Nakajima, Takuto Matsushita and Jian Ping Gong

Macromolecules, 2025, 58, 6017
DOI: 10.1021/acs.macromol.4c02446

Robust Self-Healing Magnetically Induced Colloidal Photonic Crystal Hydrogels

Su-Na Yin, Juan Liu, Defeng Wu, Su Chen and Weiwei Xia

ACS Appl. Polym. Mater., 2020, 2, 448
DOI: 10.1021/acsapm.9b00905

Facile fabrication of nonswellable and biocompatible hydrogels with cartilage-comparable performances

Chunhui Luo, Andi Guo, Yufei Zhao, Jing Sun and Zhibo Li

Materials Today Communications, 2021, 27, 102375
DOI: 10.1016/j.mtcomm.2021.102375

Network modeling of the chitin nanofiber/poly-epoxy hybrid network in the double-network hydrogel

Junchao Huang and Peng Cao

International Journal of Biological Macromolecules, 2025, 306, 141537
DOI: 10.1016/j.ijbiomac.2025.141537

Multiscale FE modeling of double-network gels with viscoelastic and anisotropic damage coupling

Lionel Ogouari, Qiang Guo, Fahmi Zaïri, Thanh-Tam Mai, Yong Zheng, Jian Ping Gong and Kenji Urayama

International Journal of Plasticity, 2026, 200, 104666
DOI: 10.1016/j.ijplas.2026.104666

Nano-hydroxyapatite enhanced double network hydrogels with excellent mechanical properties for potential application in cartilage repair

Shuchun Gan, Weinan Lin, Yongliang Zou, Bo Xu, Xiong Zhang, Jianhao Zhao and Jianhua Rong

Carbohydrate Polymers, 2020, 229, 115523
DOI: 10.1016/j.carbpol.2019.115523

Quantitative evaluation of macromolecular crowding environment based on translational and rotational diffusion using polarization dependent fluorescence correlation spectroscopy

Johtaro Yamamoto, Akito Matsui, Fusako Gan, Makoto Oura, Riku Ando, Takahiro Matsuda, Jian Ping Gong and Masataka Kinjo

Sci Rep, 2021, 11
DOI: 10.1038/s41598-021-89987-7

Mechanoresponsive self-growing hydrogels inspired by muscle training

Takahiro Matsuda, Runa Kawakami, Ryo Namba, Tasuku Nakajima and Jian Ping Gong

Science, 2019, 363, 504
DOI: 10.1126/science.aau9533

Dual-Crosslinked Gelatin/Dextran Medical Hydrogels Based on Aldimine Condensation and Photopolymerization

Xia Ding, Bing Yang, Lei Ni, Guangliang Niu, Xinyi Si, Ning Lu and Zhaosheng Hou

Gels, 2025, 11, 871
DOI: 10.3390/gels11110871

Tuning the Ultimate Strain of Single and Double Network Gels Through Reactive Strand Extension

Xujun Zheng, Chun-Yu Chiou, Sunay Dilara Ekim, Tatiana B. Kouznetsova, Jafer Vakil, Yixin Hu, Liel Sapir, Danyang Chen, Zi Wang, Michael Rubinstein, Jian Ping Gong, Nancy R. Sottos and Stephen L. Craig

ACS Cent. Sci., 2025, 11, 1882
DOI: 10.1021/acscentsci.5c00932

Necking of double-network gels: Constitutive modeling with microstructural insight

Vahid Morovati, Mohammad Ali Saadat and Roozbeh Dargazany

Phys. Rev. E, 2020, 102
DOI: 10.1103/PhysRevE.102.062501

Multifunctional Nanoengineered Hydrogels Consisting of Black Phosphorus Nanosheets Upregulate Bone Formation

Zhenming Wang, Jin Zhao, Wanze Tang, Liqiu Hu, Xin Chen, Yiping Su, Chang Zou, Jianhong Wang, William W. Lu, Wanxin Zhen, Ronghua Zhang, Dazhi Yang and Songlin Peng

Small, 2019, 15
DOI: 10.1002/smll.201901560

New Approaches to the Design of Double Polymer Networks: a Review

A. V. Shibaev and O. E. Philippova

Polym. Sci. Ser. C, 2022, 64, 26
DOI: 10.1134/S1811238222200012

Poroelastic fracture of polyacrylamide hydrogels: Enhanced crack tip swelling driven by chain scission

Qifang Zhang, Junjie Liu, Gang Zhang, Yuhong Li, Nan Hu, Jinglei Yang, Yan Yang, Shaoxing Qu, Qianhua Kan and Guozheng Kang

Journal of the Mechanics and Physics of Solids, 2025, 194, 105954
DOI: 10.1016/j.jmps.2024.105954

How chain dynamics affects crack initiation in double-network gels

Yong Zheng, Takahiro Matsuda, Tasuku Nakajima, Wei Cui, Ye Zhang, Chung-Yuen Hui, Takayuki Kurokawa and Jian Ping Gong

Proc. Natl. Acad. Sci. U.S.A., 2021, 118
DOI: 10.1073/pnas.2111880118

Effect of crosslinking on the mechanical properties of multiple network elastomers: experiments and modeling

Ning Han, Peng Sun, Danming Zhong, Rui Xiao and Shaoxing Qu

Acta Mech. Sin., 2026, 42
DOI: 10.1007/s10409-025-25414-x

Proteoglycans and Glycosaminoglycans Improve Toughness of Biocompatible Double Network Hydrogels

Yu Zhao, Tasuku Nakajima, Jing Jing Yang, Takayuki Kurokawa, Jian Liu, Jishun Lu, Shuji Mizumoto, Kazuyuki Sugahara, Nobuto Kitamura, Kazunori Yasuda, A. U. D. Daniels and Jian Ping Gong

Advanced Materials, 2014, 26, 436
DOI: 10.1002/adma.201303387

On mechanical properties of nanocomposite hydrogels: Searching for superior properties

Wenjin Xing and Youhong Tang

Nano Materials Science, 2022, 4, 83
DOI: 10.1016/j.nanoms.2021.07.004

Biomedical applications of stimuli-responsive “smart” interpenetrating polymer network hydrogels

Jiuping Wu, Wu Xue, Zhihe Yun, Qinyi Liu and Xinzhi Sun

Materials Today Bio, 2024, 25, 100998
DOI: 10.1016/j.mtbio.2024.100998

An anisotropic damage model for the mechanical and chemo-mechanical coupling behaviors of double-network hydrogels

Ning Han, Peng Sun, Jinye Zhu, Rui Xiao, Shaoxing Qu and Danming Zhong

International Journal of Solids and Structures, 2026, 333, 113962
DOI: 10.1016/j.ijsolstr.2026.113962

4D Printing with Mechanically Robust, Thermally Actuating Hydrogels

Shannon E. Bakarich, Robert Gorkin, Marc in het Panhuis and Geoffrey M. Spinks

Macromol. Rapid Commun., 2015, 36, 1211
DOI: 10.1002/marc.201500079

Fracture mechanics of a self-healing hydrogel with covalent and physical crosslinks: A numerical study

Jingyi Guo, Mincong Liu, Alan T. Zehnder, Jingwen Zhao, Tetsuhara Narita, Costantino Creton and Chung-Yuen Hui

Journal of the Mechanics and Physics of Solids, 2018, 120, 79
DOI: 10.1016/j.jmps.2018.03.009

Enhanced adhesion strength of polyacrylamide-tannic hydrogel to concrete surface through reactive particle aggregation of calcium aluminate cement

Shuaizu Gu, Yuan Hu, Dandan Sun, Jingwen Wang, Pan Feng, Junyuan Guo, Linglin Xu and Kai Wu

Composites Communications, 2025, 58, 102515
DOI: 10.1016/j.coco.2025.102515

Highly strong and sensitive bilayer hydrogel actuators enhanced by cross-oriented nanocellulose networks

Wei Liu, Lihong Geng, Jianming Wu, An Huang and Xiangfang Peng

Composites Science and Technology, 2022, 225, 109494
DOI: 10.1016/j.compscitech.2022.109494

Tough and pH-sensitive hydroxypropyl guar gum/polyacrylamide hybrid double-network hydrogel

Jingjing Zhu, Shuang Guan, Qianqian Hu, Guanghui Gao, Kun Xu and Pixin Wang

Chemical Engineering Journal, 2016, 306, 953
DOI: 10.1016/j.cej.2016.08.026

A variable stiffness robotic gripper with soft revolute joint composed of double-network gel

Moses Gladson Selvamuthu, Kazunari Yoshida, Hidemitsu Furukawa and Riichiro Tadakuma

Advanced Robotics, 2025, 39, 1463
DOI: 10.1080/01691864.2025.2586784

Hydrogel wound dressings for bioactive treatment of acute and chronic wounds

Julia Koehler, Ferdinand P. Brandl and Achim M. Goepferich

European Polymer Journal, 2018, 100, 1
DOI: 10.1016/j.eurpolymj.2017.12.046

A Review of Physically Based and Thermodynamically Based Constitutive Models for Soft Materials

Yuhai Xiang, Danming Zhong, Stephan Rudykh, Haofei Zhou, Shaoxing Qu and Wei Yang

Journal of Applied Mechanics, 2020, 87
DOI: 10.1115/1.4047776

Analysis of Fatigue Crack Nucleation in Double-Network Hydrogels

Shan Gao and Liying Jiang

Polymers, 2024, 16, 1700
DOI: 10.3390/polym16121700

Highly Stretchable and Highly Resilient Polymer–Clay Nanocomposite Hydrogels with Low Hysteresis

Xing Su, Suntharavathanan Mahalingam, Mohan Edirisinghe and Biqiong Chen

ACS Appl. Mater. Interfaces, 2017, 9, 22223
DOI: 10.1021/acsami.7b05261

Spatial Analysis of the Damage Zone in Double Network Hydrogel Using the Microelectrode Technique

Takuya Nishimura, Honglei Guo, Yoshinori Katsuyama, Masahiro Yoshida, Jian Ping Gong and Takayuki Kurokawa

Macromolecules, 2024, 57, 1502
DOI: 10.1021/acs.macromol.3c02500

Cartilage-Inspired Inhomogeneous Salt-Hydrogel for Hydrated Drag-Reducing and Strain Sensing

Yonggan Yan, Yanping Shi, Chenghu Liu, Jinlong Shao, Nengzhe Sun, Baojin Ma, Yuan Li, Jun Huang and Shaohua Ge

ACS Appl. Mater. Interfaces, 2023, 15, 48632
DOI: 10.1021/acsami.3c10271

Tensile Behaviors of Double Network Hydrogels with Varied First Network Topological and Chemical Structures

Feixue Lu, Tasuku Nakajima, Yong Zheng, Hailong Fan and Jian Ping Gong

Macromolecules, 2024, 57, 11520
DOI: 10.1021/acs.macromol.4c02087

Effect of Predamage on the Fracture Energy of Double-Network Hydrogels

Yong Zheng, Yiru Wang, Tasuku Nakajima and Jian Ping Gong

ACS Macro Lett., 2024, 130
DOI: 10.1021/acsmacrolett.3c00702

Highly stretchable covalent adaptive networks enabled by dynamic boronic diester linkages with nitrogen→boron coordination

Zhenyu Lyu, Shiqi Sun and Tongfei Wu

Journal of Polymer Science, 2022, 60, 72
DOI: 10.1002/pol.20210706

Self-Healable, Tough, and Ultrastretchable Nanocomposite Hydrogels Based on Reversible Polyacrylamide/Montmorillonite Adsorption

Guorong Gao, Gaolai Du, Yuanna Sun and Jun Fu

ACS Appl. Mater. Interfaces, 2015, 7, 5029
DOI: 10.1021/acsami.5b00704

Marked Sensitivity of Ultimate Elongation to Loading Axiality in Polyrotaxane Gels with Largely Slidable Cross Links

Takuma Aoyama, Kazuaki Kato and Kenji Urayama

ACS Macro Lett., 2022, 11, 362
DOI: 10.1021/acsmacrolett.1c00801

Crystallization‐Induced Network Growth for Enhancing Hydrogel Mechanical Properties

Qianwei Liu, Xinhong Xiong, Yuanlai Fang and Jiaxi Cui

Small, 2025, 21
DOI: 10.1002/smll.202500976

Fracture Process of Microgel-Reinforced Hydrogels under Uniaxial Tension

Jian Hu, Takayuki Kurokawa, Tasuku Nakajima, Zi Liang Wu, Song Miao Liang and Jian Ping Gong

Macromolecules, 2014, 47, 3587
DOI: 10.1021/ma5008545

Ductility, toughness and strain recovery in self-healing dual cross-linked nanoparticle networks studied by computer simulations

Balaji V.S. Iyer, Victor V. Yashin, Matthew J. Hamer, Tomasz Kowalewski, Krzysztof Matyjaszewski and Anna C. Balazs

Progress in Polymer Science, 2015, 40, 121
DOI: 10.1016/j.progpolymsci.2014.07.004

Natural Phytic Acid-Assisted Polyaniline/Poly(vinyl alcohol) Hydrogel Showing Self-Reinforcing Features

Lianjie Zhao, Hao Zhang, Ning Tang, Min-Hui Li and Jun Hu

ACS Appl. Mater. Interfaces, 2023, 15, 41927
DOI: 10.1021/acsami.3c09032

Thermodynamically stable whilst kinetically labile coordination bonds lead to strong and tough self-healing polymers

Jian-Cheng Lai, Xiao-Yong Jia, Da-Peng Wang, Yi-Bing Deng, Peng Zheng, Cheng-Hui Li, Jing-Lin Zuo and Zhenan Bao

Nat Commun, 2019, 10
DOI: 10.1038/s41467-019-09130-z

Regulating cyclic behaviors of tough soft materials: A generic, mechanism-based damage model approach

Peng Xu, Pingping Zhu, Yongzhi Liang and Zheng Zhong

International Journal of Solids and Structures, 2026, 325, 113699
DOI: 10.1016/j.ijsolstr.2025.113699

Molecular weight distribution of network strands in double network hydrogels estimated by mechanical testing

Hai Xin, Hugh R. Brown and Geoffrey M. Spinks

Polymer, 2014, 55, 3037
DOI: 10.1016/j.polymer.2014.05.005

Large deformation effect in Mode I crack opening displacement of an Agar gel: A comparison of experiment and theory

Rong Long, Maxime Lefranc, Elisabeth Bouchaud and Chung-Yuen Hui

Extreme Mechanics Letters, 2016, 9, 66
DOI: 10.1016/j.eml.2016.05.005

A Constitutive Model for Soft Materials Incorporating Viscoelasticity and Mullins Effect

Tongqing Lu, Jikun Wang, Ruisen Yang and T. J. Wang

Journal of Applied Mechanics, 2017, 84
DOI: 10.1115/1.4035180

Injectable and Cytocompatible Tough Double‐Network Hydrogels through Tandem Supramolecular and Covalent Crosslinking

Christopher B. Rodell, Neville N. Dusaj, Christopher B. Highley and Jason A. Burdick

Advanced Materials, 2016, 28, 8419
DOI: 10.1002/adma.201602268

Rate dependent fracture of hydrogels: from small to large-scale swelling

Yan Yang, Tongqing Lu and Tiejun Wang

Acta Mech. Sin., 2025, 41
DOI: 10.1007/s10409-025-25166-x

Molecular mechanism of abnormally large nonsoftening deformation in a tough hydrogel

Ya Nan Ye, Kunpeng Cui, Wei Hong, Xueyu Li, Chengtao Yu, Dominique Hourdet, Tasuku Nakajima, Takayuki Kurokawa and Jian Ping Gong

Proc. Natl. Acad. Sci. U.S.A., 2021, 118
DOI: 10.1073/pnas.2014694118

Characterization of fracture toughness and damage zone of double network hydrogels

Yetong Jia, Zidi Zhou, Huilong Jiang and Zishun Liu

Journal of the Mechanics and Physics of Solids, 2022, 169, 105090
DOI: 10.1016/j.jmps.2022.105090

Double-Network Hydrogel Films Based on Cellulose Derivatives and κ-Carrageenan with Enhanced Mechanical Strength and Superabsorbent Properties

Jiseon Kang and Seok Il Yun

Gels, 2022, 9, 20
DOI: 10.3390/gels9010020

Swelling of Hydrogels With Imperfect Polymer Networks

Yan Yang and Tiejun Wang

Journal of Applied Mechanics, 2025, 92
DOI: 10.1115/1.4068317

Characterizing Large Strain Elasticity of Brittle Elastomeric Networks by Embedding Them in a Soft Extensible Matrix

Etienne Ducrot and Costantino Creton

Adv Funct Materials, 2016, 26, 2482
DOI: 10.1002/adfm.201504536

Unique crack propagation of double network hydrogels under high stretch

Ye Zhang, Kazuki Fukao, Takahiro Matsuda, Tasuku Nakajima, Katsuhiko Tsunoda, Takayuki Kurokawa and Jian Ping Gong

Extreme Mechanics Letters, 2022, 51, 101588
DOI: 10.1016/j.eml.2021.101588

Cellulosic gel-based triboelectric nanogenerators for energy harvesting and emerging applications

Ying Qin, Wanglin Zhang, Yanhua Liu, Jiamin Zhao, Jinxia Yuan, Mingchao Chi, Xiangjiang Meng, Guoli Du, Chenchen Cai, Shuangfei Wang and Shuangxi Nie

Nano Energy, 2023, 106, 108079
DOI: 10.1016/j.nanoen.2022.108079

Hydrogel morphogenesis induced by force-controlled growth

Zhi Jian Wang, Ji Lin, Tasuku Nakajima and Jian Ping Gong

Proc. Natl. Acad. Sci. U.S.A., 2024, 121
DOI: 10.1073/pnas.2402587121

Regulating Color Activation Energy of Mechanophore-Linked Multinetwork Elastomers

Wenlian Qiu, Paul A. Gurr and Greg G. Qiao

Macromolecules, 2020, 53, 4090
DOI: 10.1021/acs.macromol.0c00477

Anisotropic, Flexible Wood Hydrogels and Wrinkled, Electrodeposited Film Electrodes for Highly Sensitive, Wide-Range Pressure Sensing

Kangchen Nie, Zhaosong Wang, Ruixin Tang, Li Zheng, Caicai Li, Xiaoping Shen and Qingfeng Sun

ACS Appl. Mater. Interfaces, 2020, 12, 43024
DOI: 10.1021/acsami.0c13962

50th Anniversary Perspective: Networks and Gels: Soft but Dynamic and Tough

Costantino Creton

Macromolecules, 2017, 50, 8297
DOI: 10.1021/acs.macromol.7b01698

Regenerated Cellulose Microgel: A Promising Reinforcing Agent and Gelator for Soft Matter

Kai Li, Xin Chen, Yingchao Wang, Bin Sun, Ziting Yuan and Yuxin Liu

ACS Appl. Polym. Mater., 2021, 3, 4101
DOI: 10.1021/acsapm.1c00588

In Situ Forming, Cytocompatible, and Self-Recoverable Tough Hydrogels Based on Dual Ionic and Click Cross-Linked Alginate

Mohammad Hossein Ghanian, Hamid Mirzadeh and Hossein Baharvand

Biomacromolecules, 2018, 19, 1646
DOI: 10.1021/acs.biomac.8b00140

Characterizing dissipated energy density distribution and damage zone in double network hydrogels

Jiapeng You, Chong Wang, Zhixuan Li and Zishun Liu

Journal of the Mechanics and Physics of Solids, 2025, 196, 106006
DOI: 10.1016/j.jmps.2024.106006

Mechanics of a Dual Cross-Link Gel with Dynamic Bonds: Steady State Kinetics and Large Deformation Effects

Jingyi Guo, Rong Long, Koichi Mayumi and Chung-Yuen Hui

Macromolecules, 2016, 49, 3497
DOI: 10.1021/acs.macromol.6b00421

Fabrication of Tough and Stretchable Hybrid Double-Network Elastomers Using Ionic Dissociation of Polyelectrolyte in Nonaqueous Media

Takahiro Matsuda, Tasuku Nakajima and Jian Ping Gong

Chem. Mater., 2019, 31, 3766
DOI: 10.1021/acs.chemmater.9b00871

Metal-Coordinated Dynamics and Viscoelastic Properties of Double-Network Hydrogels

Shilei Zhu, Yan Wang, Zhe Wang, Lin Chen, Fengbo Zhu, Yanan Ye, Yong Zheng, Wenwen Yu and Qiang Zheng

Gels, 2023, 9, 145
DOI: 10.3390/gels9020145

Finite strain damage-elastoplasticity in double-network hydrogels

S. Shams Es-haghi and R.A. Weiss

Polymer, 2016, 103, 277
DOI: 10.1016/j.polymer.2016.09.054

A Review on the Mullins Effect in Tough Elastomers and Gels

Lin Zhan, Shaoxing Qu and Rui Xiao

Acta Mech. Solida Sin., 2024, 37, 181
DOI: 10.1007/s10338-023-00460-6

Polymers Resist Fatigue Crack Growth by Deconcentrating Stress

Jason Steck, Christine Heera Ahn and Zhigang Suo

Annual Review of Materials Research, 2025, 55, 333
DOI: 10.1146/annurev-matsci-101922-122133

Superhydrophilic and underwater superoleophobic hydrogel-loaded fabrics for enhanced oil/water separation

Hao Huang, Daofeng Zhu, Abbas Ahmed, Anqi Liang, Yanling Yang, Baohan He, Xiaoyan Li, Fuchuan Ding and Luyi Sun

Polymer, 2024, 306, 127174
DOI: 10.1016/j.polymer.2024.127174

Force-triggered rapid microstructure growth on hydrogel surface for on-demand functions

Qifeng Mu, Kunpeng Cui, Zhi Jian Wang, Takahiro Matsuda, Wei Cui, Hinako Kato, Shotaro Namiki, Tomoko Yamazaki, Martin Frauenlob, Takayuki Nonoyama, Masumi Tsuda, Shinya Tanaka, Tasuku Nakajima and Jian Ping Gong

Nat Commun, 2022, 13
DOI: 10.1038/s41467-022-34044-8

Unraveling bio-inspired pre-swollen effects of tetra-polyethylene glycol double network hydrogels with ultra-stretchable yielding strain

Xiaodong Wang, Haibao Lu, Nan Wu, David Hui and Yongqing Fu

Smart Mater. Struct., 2019, 28, 035005
DOI: 10.1088/1361-665X/aaf5b6

Dual Ionically Cross-linked Double-Network Hydrogels with High Strength, Toughness, Swelling Resistance, and Improved 3D Printing Processability

Xuefeng Li, Hui Wang, Dapeng Li, Shijun Long, Gaowen Zhang and ZiLiang Wu

ACS Appl. Mater. Interfaces, 2018, 10, 31198
DOI: 10.1021/acsami.8b13038

Toughening Elastomers Using a Mussel-Inspired Multiphase Design

Xuhui Zhang, Jun Liu, Zhiyu Zhang, Siwu Wu, Zhenghai Tang, Baochun Guo and Liqun Zhang

ACS Appl. Mater. Interfaces, 2018, 10, 23485
DOI: 10.1021/acsami.8b08844

Hierarchical Tough Hydrogel with Enhanced Rigidity and Extensibility for Strain Sensing, Posture Guide, and Injury‐Prevention

Nuri Park, Ziwen Fan and Jaeyun Kim

Adv Funct Materials, 2025, 35
DOI: 10.1002/adfm.202419830

Energy Dissipation and Mechanoresponsive Color Evaluation of a Poly(n-hexyl Methacrylate) Soft Material Enhanced by a Mechanochromic Cross-Linker with Dynamic Covalent Bonds

Yuchen Mao, Yuto Kubota, Takashi Kurose, Akira Ishigami, Kota Seshimo, Daisuke Aoki, Hideyuki Otsuka and Hiroshi Ito

Macromolecules, 2020, 53, 9313
DOI: 10.1021/acs.macromol.0c01770

Effects of Added Physical Cross‐Linkers on Mechanical Properties of Polymer Networks

Tsutomu Furuya, Keita Yamamoto and Tsuyoshi Koga

Macro Theory & Simulations, 2019, 28
DOI: 10.1002/mats.201800042

Advanced Functional Polymers: Properties and Supramolecular Phenomena in Hydrogels and Polyrotaxane-based Materials

Abu Bin Ihsan, Abu Bin Imran and Md. Abu Bin Hasan Susan

Chemistry Africa, 2023, 6, 79
DOI: 10.1007/s42250-022-00460-y

A double network hydrogel with high mechanical strength and shape memory properties

Lei Zhu, Chun-ming Xiong, Xiao-fen Tang, Li-jun Wang, Kang Peng and Hai-yang Yang

Chinese Journal of Chemical Physics, 2018, 31, 350
DOI: 10.1063/1674-0068/31/cjcp1710188

A Multiaxial Theory of Double Network Hydrogels

Vu Ngoc Khiêm, Thanh-Tam Mai, Kenji Urayama, Jian Ping Gong and Mikhail Itskov

Macromolecules, 2019, 52, 5937
DOI: 10.1021/acs.macromol.9b01044

Stretch-induced softening in filled elastomers: A review on Mullins effect related anisotropy and thermally induced recovery

Isabella Denora and Claudia Marano

Polymer Testing, 2024, 133, 108399
DOI: 10.1016/j.polymertesting.2024.108399

Mechanical recoverability and damage process of ionic‐covalent PAAm‐alginate hybrid hydrogels

Hai Xin, Hugh R. Brown, Sina Naficy and Geoffrey M. Spinks

J Polym Sci B Polym Phys, 2016, 54, 53
DOI: 10.1002/polb.23899

Multi‐scale modeling of double network hydrogels

İsmail Doğan Külcü, Roozbeh Dargazany and Mikhail Itskov

Proc Appl Math and Mech, 2014, 14, 391
DOI: 10.1002/pamm.201410183

Stimuli-Responsive Transformation of a Gradient Gel

Tasuku NAKAJIMA, Kenta HIWATASHI, Jian HU, Takayuki KUROKAWA and Jian Ping GONG

KOBUNSHI RONBUNSHU, 2017, 74, 311
DOI: 10.1295/koron.2017-0012

In Situ and Real-Time Visualization of Mechanochemical Damage in Double-Network Hydrogels by Prefluorescent Probe via Oxygen-Relayed Radical Trapping

Yong Zheng, Julong Jiang, Mingoo Jin, Daiyo Miura, Fei Xue Lu, Koji Kubota, Tasuku Nakajima, Satoshi Maeda, Hajime Ito and Jian Ping Gong

J. Am. Chem. Soc., 2023, 145, 7376
DOI: 10.1021/jacs.2c13764

The fracture and toughening mechanism of double-network hydrogel using the network mechanics method

Han Li, Jincheng Lei, Danyang Wang and Zishun Liu

Engineering Fracture Mechanics, 2024, 309, 110413
DOI: 10.1016/j.engfracmech.2024.110413