Electrocatalytic CO2 Reduction with an Immobilized Iron Complex on Gas Diffusion Electrodes
Abstract
The immobilization of molecular electrocatalysts on gas diffusion electrodes (GDEs) overcomes mass transport limitations inherent to solution-phase CO2 reduction. We report the immobilization of the molecular FeTDHPP catalyst on a GDE via supramolecular π-π interactions, achieving a 50-fold catalytic activity increase compared to solution-phase performance.
- This article is part of the themed collection: Chemistry at the Forefront of the Sustainable Energy Transition