MAPI–MoS2 quantum dot composite films as active layers for efficient photovoltaics

Abstract

In this work we have incorporated MoS₂ quantum dots having outstanding optoelectronic properties with methyl ammonium lead iodide (MAPI) to form a composite absorber material for photovoltaic applications. The inclusion of MoS₂ quantum dots in the perovskite layer improves the absorption and charge transport properties of the active layer, in part due to the quantum dots contributing to defect passivation at the MAPI grain interfaces. The photocurrent density increases when the MoS₂ quantum dots are introduced in the device structure, resulting in efficiency improvements of 14% and 28% for devices fabricated in different laboratories.