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Org. Chem. Front., 2015, Advance Article
DOI: 10.1039/C5QO00236B, Research Article
Novel pincer-type N-heterocyclic carbene ligands have been synthesised and characterised by FAB-MS and single crystal X-ray analysis. The ligands have proved to be highly active towards palladium-catalysed Suzuki–Miyaura cross-coupling of bromoanthracene and related substrates.
 
Org. Chem. Front., 2015, Accepted Manuscript
DOI: 10.1039/C5QO00155B, Research Article
The ortho- and meta-substituted NHC-oxazoline ligands based on phenyl scaffold have been synthesized in a six-step pathway, and their coordination with Au(Me2S)Cl gave the corresponding NHC-gold(I) complexes in good yields....
 
Org. Chem. Front., 2015, Accepted Manuscript
DOI: 10.1039/C5QO00220F, Research Article
A novel visible-light-induced alkene difunctionalization strategy is described for the synthesis of 1,5-dicarbonyl compounds from two reaction partners, α-aryl allylic alcohols and α-carbonyl alkyl bromides. This method is successful by...
 
Org. Chem. Front., 2015, Accepted Manuscript
DOI: 10.1039/C5QO00219B, Research Article
An unprecedented silver-catalyzed 1,3-dipolar cycloaddition reaction of isocyanides with diazo compounds to afford 1,4-disubstituted 1,2,3-triazoles was reported. This reaction exhibits remarkable features, such as high regioselectivity, mild reaction conditions, easily...
 
Org. Chem. Front., 2015, Advance Article
DOI: 10.1039/C5QO00224A, Tutorial Account
We herein summarize recent Ni-catalyzed reductive coupling of alkyl electrophiles with a variety of other electrophiles to generate C(sp3)–C(sp3) and C(sp3)–C(sp2) bonds.
 
Avanashiappan Nandakumar, Manoj K. Sahoo and Ekambaram Balaraman
Org. Chem. Front., 2015, Advance Article
DOI: 10.1039/C5QO00229J, Highlight
Recent progress in transition-metal catalysed acceptor- and acceptorless-reverse hydroformylation of aldehydes for the conversion of olefins has been discussed. The aldehyde feedstock serves as a source for production of syngas and valuable alkenes.
 
Fangdong Hu, Jinghui Yang, Ying Xia, chen ma, Haiping Xia, Yan Zhang and Jianbo Wang
Org. Chem. Front., 2015, Accepted Manuscript
DOI: 10.1039/C5QO00241A, Research Article
Cross-coupling of N-tosylhydrazones with chromium Fischer carbene complexes under catalyst-free conditions have been developed. This protocol is featured by taking advantage of stable carbene complexes and reactive diazo compounds, which...
 
Mariwan A. Hama Salih, Louise Male, Neil Spencer and John S. Fossey
Org. Chem. Front., 2015, Advance Article
DOI: 10.1039/C5QO00183H, Research Article
1,3,5-Substituted pyrrolidin-2-ones were synthesised via an iodine mediated cyclisation of 3-methyl substituted homoallylamines in good to excellent yield, as mixtures of diastereoisomers. Furan bispyrrolidines were formed as single diastereoisomers when 3-phenyl homoallylamines were employed in an analogous reaction.
 
Yuan Jiang, Linan Yang, Christine M. Bohn, Guannan Li, Dong Han, Nathan S. Mosier, Jeffrey T. Miller, Hilkka I. Kenttämaa and Mahdi M. Abu-Omar
Org. Chem. Front., 2015, Advance Article
DOI: 10.1039/C5QO00194C, Research Article
Identification of catalytic species and their contributions in iron catalyzed sugar conversion to hydroxymethylfurfural and levulinic acid.
 
En-Jian Han, Yan Sun, Qian Shen, Qing-Yun Chen, Yong Guo and Yan-Gen Huang
Org. Chem. Front., 2015, Advance Article
DOI: 10.1039/C5QO00210A, Research Article
Cu-Promoted coupling reactions of HCFC-123 with terminal alkynes give trifluoroethylated internal alkynes.
 
Org. Chem. Front., 2015, Advance Article
DOI: 10.1039/C5QO00230C, Review Article
This review summarizes 50 years of attempts to observe, and finally isolate, the elusive oxyallyl derivatives.
 
Org. Chem. Front., 2015, Advance Article
DOI: 10.1039/C5QO00207A, Research Article
Fused β-carbolines were synthesized via a visible light photoredox catalyzed oxidation/[3 + 2] cycloaddition/oxidative aromatization reaction cascade in batch and flow microreactors.
 
Ye-Xing Lao, Jia-Qiang Wu, Yunyun Chen, Shang-Shi Zhang, Qingjiang Li and Honggen Wang
Org. Chem. Front., 2015, Advance Article
DOI: 10.1039/C5QO00218D, Research Article
A palladium-catalyzed C(sp3)–H arylation of adamantane at the methylene position with the assistance of an amide group was developed.
 
Org. Chem. Front., 2015, Advance Article
DOI: 10.1039/C5QO00203F, Research Article
Pd(II)-catalyzed, Cu(II)-mediated indole synthesis from pyrroles and 3-chloropropiophenones has been efficiently achieved. In-situ generated enones were employed for the establishment of a benzene ring onto a pyrrole backbone via dehydrochlorination/C–H olefination/cycloaddition/dehydrogenative aromatization.
 
Chuanling Song, Yihua Sun, Jianwu Wang, Hui Chen, Jiannian Yao, Chen-Ho Tung and Zhenghu Xu
Org. Chem. Front., 2015, Advance Article
DOI: 10.1039/C5QO00205B, Research Article
A new and efficient strategy for the synthesis of tetraaryl-substituted olefins with two cis furans based on a Cu/Pd catalyzed oxidative coupling reaction of cyclopropene with internal alkyne was developed. These novel tetraarylethenes were fully characterized and proved to be good AIE luminogens.
 
Chunli Liu, Minghui Zhu, Wei Wei, Daoshan Yang, Hong Cui, Xiaoxia Liu and Hua Wang
Org. Chem. Front., 2015, Advance Article
DOI: 10.1039/C5QO00208G, Research Article
A novel and efficient procedure for direct difunctionalization of alkenes with I2O5 and P(O)–H compounds has been developed under metal-free conditions.
 
Org. Chem. Front., 2015, Advance Article
DOI: 10.1039/C5QO00226E, Review Article
Asymmetric catalysis has grown rapidly and made considerable progress in the last few decades, but there still remain significantly unachievable reactions through either organocatalysis or transition-metal catalysis alone.
 
Org. Chem. Front., 2015, Advance Article
DOI: 10.1039/C5QO00187K, Research Article
A chemoselective and fast decarboxylative allylation is developed by photoredox catalysis to build C(sp3)–allyl bonds under mild conditions.
 
Org. Chem. Front., 2015, Advance Article
DOI: 10.1039/C5QO00196J, Research Article
Acrylamidines were synthesized via the copper-catalyzed three-component reaction of propargyl acetates, sulfonyl azides and amines, which are readily accessible materials.
 
Org. Chem. Front., 2015, Advance Article
DOI: 10.1039/C5QO00142K, Research Article
A series of P-chiral biaryl phosphonates were efficiently synthesized from diaryl 2-bromo arylphosphonates in high yields (up to 92%) and good enantioselectivities (up to 88% ee) through a palladium-catalyzed desymmetric intramolecular cyclization with a P-chiral biaryl monophosphorus ligand.
 
Org. Chem. Front., 2015, Advance Article
DOI: 10.1039/C5QO00179J, Research Article
An efficient approach for organoselenium-catalyzed synthesis of indoles via intramolecular C–H amination has been developed.
 
Org. Chem. Front., 2015, Advance Article
DOI: 10.1039/C5QO00150A, Research Article
An efficient method for the construction of 2-aminobenzo[d][1,3]selenazines under metal-free conditions was established.
 
Org. Chem. Front., 2015, Advance Article
DOI: 10.1039/C5QO00202H, Research Article
An efficient protocol for the synthesis of the Passerini adducts α-acyloxycarboxamides from aldehydes, isocyanides and water in a molecular ratio of 3 : 1 : 3 was described.
 
Org. Chem. Front., 2015, Advance Article
DOI: 10.1039/C5QO00148J, Research Article
An efficient asymmetric nickel-catalyzed alkylative alkyne–aldehyde cross-coupling is developed by employing BI-DIME as the P-chiral monophosphorus ligand, allowing rapid access to a series of chiral tetra-substituted olefinic allylic alcohols in high yields and good to excellent ees.
 
Org. Chem. Front., 2015, Advance Article
DOI: 10.1039/C5QO00112A, Research Article
Practical synthesis of β-alkyl α-amino acids via C(sp3)–H alkylation at room temperature.
 

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