Journal cover: Organic Chemistry Frontiers

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Org. Chem. Front., 2015, Advance Article
DOI: 10.1039/C4QO90045F, Conference Report
The CASE 2014 symposium: catalysis and sensing for our environment, Xiamen 7th–9th November 2014
 
Org. Chem. Front., 2015, Advance Article
DOI: 10.1039/C4QO00300D, Research Article
A direct carboxylation reaction of allylic bromides mediated by zinc powder with 1 atm of CO2 provided by a balloon has been developed. The reaction occurred smoothly at room temperature in the presence of LiOAc with an excellent branched regioselectivity.
 
Org. Chem. Front., 2015, Advance Article
DOI: 10.1039/C4QO00207E, Review Article
This review is focused on the recent advances in the transition metal-catalyzed direct remote C–H-functionalization of alkyl groups via C(sp3)–H bond activation. In general, carboxamide/ester-chelated β-functionalization reactions are summarized.
 
Org. Chem. Front., 2015, Advance Article
DOI: 10.1039/C4QO90043J, Editorial
Meet the Advisory Board of Organic Chemistry Frontiers
 
Org. Chem. Front., 2015, Advance Article
DOI: 10.1039/C4QO00293H, Research Article
An organocatalytic approach for the synthesis of isochroman derivatives via direct C(sp3)–H bond and N–H bond coupling is described. The C–N (amine or amide) and C[double bond, length as m-dash]N (imidate) products can be selectively achieved by controlling the amount of oxidants.
 
Org. Chem. Front., 2015, Advance Article
DOI: 10.1039/C4QO90044H, Profile
Meet Professor Guy Bertrand, from the University of California San Diego (USA).
 
Org. Chem. Front., 2014, Accepted Manuscript
DOI: 10.1039/C4QO00276H, Research Article
From themed collection Celebrating the 80th Birthday of Professor Ei-ichi Negishi
A copper(II)-catalyzed methoxylation of unactivated (hetero)aryl C-H bonds directed by our newly developed PIP directing group with methanol has been achieved. This protocol occurs efficiently with catalytic amount of copper...
 
Org. Chem. Front., 2015, Advance Article
DOI: 10.1039/C4QO00287C, Research Article
13-Vertex closo-carboranes and N-heterocyclic carbenes undergo a fast acid–base reaction to generate intermediates that are slowly converted to the final products.
 
Org. Chem. Front., 2014, Accepted Manuscript
DOI: 10.1039/C4QO00291A, Tutorial Account
This tutorial account describes a robust carbonyl gem-difluoroolefination reagent, the difluoromethyl 2-pyridyl sulfone, developed in our group recently. Guidelines for its laboratory preparation and applications are presented in details for...
 
Yi-Xia Jia, Hao Wu, Ren-Rong Liu, Chong Shen, Min-Di Zhang and Jianrong Gao
Org. Chem. Front., 2014, Accepted Manuscript
DOI: 10.1039/C4QO00265B, Research Article
Using Ni(ClO4)2−bisoxazoline complex as a catalyst, the enantioselective Friedel−Crafts alkylation of 4,7-dihydroindoles with β-CF3-β-disubstituted nitroalkenes was furnished in high enantioselectivities (up to 91%) to give alkylated dihydroindoles bearing trifluoromethylated all-carbon...
 
Org. Chem. Front., 2014, Accepted Manuscript
DOI: 10.1039/C4QO00294F, Review Article
1,2,3,4-Tetrahydroisoquinoline is one of the most important “privileged scaffolds” present in natural products. C1-chiral tetrahydroisoquinolines have exhibited a wide variety of bioactivities and found applications as chiral scaffolds in asymmetric...
 
Zhiyong Wang, Lin Tang, Yu Yang, Lixian Wen, Sheng Zhang and Zhenggen Zha
Org. Chem. Front., 2014, Accepted Manuscript
DOI: 10.1039/C4QO00278D, Research Article
A highly efficient and selective nitrogen source-promoted reaction for the synthesis of 2,4-disubstituted quinazolines from o-nitroacetophenones and alcohols catalyzed by Au/TiO2 has been developed via a hydrogen-transfer strategy. This reaction...
 
Machiko Ie, Jun-ichiro Setsune, Kazuo Eda and Akihiko Tsuda
Org. Chem. Front., 2015, Advance Article
DOI: 10.1039/C4QO00268G, Research Article
From themed collection Celebrating the 80th Birthday of Professor Ei-ichi Negishi
A cyclic octapyrrole shows a strong chiroptical response upon complexation with an oligonucleotide that has high thymine content.
 
Org. Chem. Front., 2014, Accepted Manuscript
DOI: 10.1039/C4QO00306C, Review Article
In this minireview, catalytically enantioselecitve transformations via visible light photocatalysis are discussed. High enantioselectivities are achieved in the combination of visible light photocatalysis with chiral organocatalysts. Considering the huge progress...
 
Org. Chem. Front., 2015, Advance Article
DOI: 10.1039/C4QO00282B, Research Article
The direct amidation of dipeptides through direct aryl C–H transformation of the phenylalanine residue via Pd catalysis.
 
Org. Chem. Front., 2015, Advance Article
DOI: 10.1039/C4QO00273C, Research Article
The efficient synthesis of highly functionalized furan derivatives from 1-sulfonyl-1,2,3-triazoles with a pendent carbonyl group is reported. The process involves an intramolecular trapping of α-imino carbene and subsequent aromatization.
 
Org. Chem. Front., 2015, Advance Article
DOI: 10.1039/C4QO00272E, Highlight
Recent advances in chromium-catalyzed cross-couplings of C–X and C–H bonds with Grignard reagents are highlighted.
 
Org. Chem. Front., 2015, Advance Article
DOI: 10.1039/C4QO00271G, Research Article
The asymmetric boron conjugate addition onto α,β-unsaturated ketones and esters has been developed by using the CuOTf/Josiphos complex as the catalyst under non-alkaline conditions.
 
Org. Chem. Front., 2015, Advance Article
DOI: 10.1039/C4QO00245H, Review Article
The highly efficient asymmetric reactions of chiral sulfinyl auxiliary, diene ligands and sulfur–olefin ligands are presented.
 
shoufeng wang, Qingfei Zheng, Jianfeng Wang, Zhi-Xiong Zhao, Qingye Li, Yunsong Yu, Ren-Xiao Wang and Wen Liu
Org. Chem. Front., 2014, Accepted Manuscript
DOI: 10.1039/C4QO00288A, Research Article
Thiostrepton is a potent archetypal thiopeptide antibiotic. According to its mechanism known to target bacterial ribosome, we show rational design upon modeling of this molecule into the ribosome complex and...
 
Org. Chem. Front., 2015, Advance Article
DOI: 10.1039/C4QO90042A, Editorial
Welcome to the first issue of Organic Chemistry Frontiers 2015
 
Org. Chem. Front., 2015, Advance Article
DOI: 10.1039/C4QO00246F, Research Article
The first example of Pd-catalyzed aryldifluoromethylation of arylboronic acids with readily available aryldifluoromethyl bromides has been described. Preliminary mechanistic studies revealed that a Pd(0)Ln-initiated single electron transfer (SET) pathway is involved in the catalytic cycle.
 
Jing-Rui Zhao, Xiaolong Yuan, Zhaoyan Wang, Shiwu Chen, Zhan-Xin Zhang and Weihua Xue
Org. Chem. Front., 2015, Advance Article
DOI: 10.1039/C4QO00255E, Research Article
Functional group tolerance under mild conditions eliminates the need for base additives or hygroscopic promoters.
 
Org. Chem. Front., 2015, Advance Article
DOI: 10.1039/C4QO00248B, Research Article
From themed collection Celebrating the 80th Birthday of Professor Ei-ichi Negishi
Oxidative C–H amination has proved to be an efficient strategy to construct pyrido[2′,1′:2,3]imidazo[4,5-b]indoles and their π-expanded analogs.
 

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