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Journal cover: Organic Chemistry Frontiers

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Impact Factor Pending 12 Issues per Year Free access available
 
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Org. Chem. Front., 2016, Accepted Manuscript
DOI: 10.1039/C5QO00412H, Research Article
Visible light catalytic cross coupling reaction from two different C-H bonds provides an efficient protocol for C-H bond activation and C-C bond construction. The application of oxidative photoredox strategy to...
 
Org. Chem. Front., 2016, Accepted Manuscript
DOI: 10.1039/C5QO00433K, Research Article
The double-mutant strain Streptomyces laurentii △tsrB/T was designed and constructed based on recent understanding regarding the structure-activity relationship between the side ring and tail of thiostrepton (TSR). Five new C-terminally...
 
Org. Chem. Front., 2016, Accepted Manuscript
DOI: 10.1039/C6QO00002A, Research Article
Density functional theory (DFT) calculations were carried out to investigate the hydridic character of several main group hydrides. A P-hydrido-1,3,2-diazaphospholene 1f with two -electron donor amino groups on the heterocyclic...
 
Org. Chem. Front., 2016, Advance Article
DOI: 10.1039/C5QO00428D, Research Article
The first asymmetric conjugate addition of diaryloxazolidin-2,4-diones to nitroolefins using an L-threonine-based tertiary amine-urea catalyst has been developed.
 
Org. Chem. Front., 2016, Accepted Manuscript
DOI: 10.1039/C5QO00402K, Research Article
The mechanism of the ring contraction reaction of (η4-1,2-disilacyclohexadiene)iron tricarbonyls was studied at the M06/LACVP* level. The Si‒Si bond of (η4-1,2-disilacyclohexadiene)iron tricarbonyls 1 was initially broken to form a η4-intermediate...
 
Org. Chem. Front., 2016, Advance Article
DOI: 10.1039/C6QO00005C, Research Article
From themed collection 2015 Emerging Investigators by OCF
An efficient palladium-catalyzed phosphonyldifluoromethylation of alkenes with bromodifluoromethylphosophonate is described. The method provides a facile access to a series of phosphonyldifluoromethylated alkenes that are of interest in medicinal chemistry. Mechanistic studies reveal that a phosphonyl difluouromethyl radical is involved in the reaction.
 
Org. Chem. Front., 2016, Accepted Manuscript
DOI: 10.1039/C5QO00437C, Highlight
This highlight describes the recent emergence of photoredox/nickel dual catalysis to generate carbon-carbon and carbon-heteroatom bonds. To address the challenges in traditional nickel-catalyzed couplings, the application of photoredox catalysis facilitates...
 
Chandrababu Naidu Kona, Mahesh N. Patil and Chepuri V. Ramana
Org. Chem. Front., 2016, Advance Article
DOI: 10.1039/C5QO00397K, Research Article
A simple procedure for the preparation of 3-(hetero)arylpropionaldehydes has been developed employing a gold-catalyzed [1,3]-rearrangement of vinyl ethers.
 
Org. Chem. Front., 2016, Advance Article
DOI: 10.1039/C5QO00432B, Research Article
From themed collection 2015 Emerging Investigators by OCF
A simple and efficient visible-light promoted intermolecular haloamination and haloetherification of alkenes was reported.
 
Org. Chem. Front., 2016, Advance Article
DOI: 10.1039/C5QO00398A, Highlight
From themed collection 2015 Emerging Investigators by OCF
Fluorinated solvents like 1,1,1,3,3,3-hexafluoroisopropanol (HFIP) and trifluoroethanol (TFE) have recently emerged as a remarkable synthetic hint allowing challenging C–H activation reactions.
 
Org. Chem. Front., 2016, Advance Article
DOI: 10.1039/C5QO00426H, Research Article
From themed collection 2015 Emerging Investigators by OCF
Co-catalyzed sequential hydroborations of alkyl and aryl alkynes with pinacolborane produce 1,1-diboronate esters with high selectivity and yields.
 
Yi-Long Zhu, De-Cai Wang, Bo Jiang, Wen-Juan Hao, Ping Wei, Ai-Fang Wang, Jiang-Kai Qiu and Shu-Jiang Tu
Org. Chem. Front., 2016, Advance Article
DOI: 10.1039/C5QO00430F, Research Article
A new metal-free oxidative hydrophosphinylation of 1,7-enynes for forming polyfunctionalized 3,4-dihydroquinolin-2(1H)-ones has been realized using readily accessible diarylphosphine oxide and TBPB as an oxidant.
 
Yucheng Mu, Xiaodong Tan, Yemin Zhang, Xiaobi Jing and Zhuangzhi Shi
Org. Chem. Front., 2016, Advance Article
DOI: 10.1039/C5QO00438A, Research Article
From themed collection 2015 Emerging Investigators by OCF
A Pd(II)-catalyzed selective β-arylation of O-methyl ketoximes was developed using iodoarenes as the coupling partners.
 
Wen-Juan Shi, Xiao-Lei Li, Zhao-Wei Li and Zhang-Jie Shi
Org. Chem. Front., 2016, Advance Article
DOI: 10.1039/C5QO00395D, Research Article
The mild Ni-catalyzed reduction of arenols features a broad substrate scope, non-sensitivity to steric hindrance and no over-reduction of the aryl ring.
 
Yu Sun, Zhanchao Meng, Pengxi Chen, Deliang Zhang, Martin Baunach, Christian Hertweck and Ang Li
Org. Chem. Front., 2016, Advance Article
DOI: 10.1039/C5QO00416K, Research Article
From themed collection 2015 Emerging Investigators by OCF
A ten-step (the longest linear sequence) total synthesis of sespenine was accomplished.
 
Org. Chem. Front., 2016, Advance Article
DOI: 10.1039/C5QO00399G, Research Article
A copper(I)-catalyzed three-component reaction of triethoxysilanes, DABCO·(SO2)2, and alkyl halides is reported. This transformation provides a facile route to sulfones under ligand-free conditions catalyzed by copper(I) oxide. The insertion of sulfur dioxide is efficient, and both triethoxyarylsilanes and triethoxyalkylsilanes are practicable during the coupling process.
 
Org. Chem. Front., 2016, Advance Article
DOI: 10.1039/C5QO00394F, Research Article
A transition-metal-free conversion of 2-arylindoles to 2-aminoarylphenones, using environmentally benign O2 as the sole oxidant, has been developed. This novel oxidative dearomatization process involves cleavage of two C–C and one C–N bonds followed by new C–C and C–O bond formation.
 
Org. Chem. Front., 2016, Advance Article
DOI: 10.1039/C5QO00392J, Research Article
From themed collection 2015 Emerging Investigators by OCF
A metal-free, photo-induced C–C bond formation methodology was developed to construct tetrahydrofluorenones and their related structures.
 
Org. Chem. Front., 2016, Advance Article
DOI: 10.1039/C5QO00387C, Research Article
A rhodium-catalyzed oxidative annulation of N-acyl anilines with alkynes was developed by using the acylamino group as a traceless directing group for the first time.
 
Zhiguo Zhang, Jingjing Qian, Guisheng Zhang, Nana Ma, Qingfeng Liu, Tongxin Liu, Kai Sun and Lei Shi
Org. Chem. Front., 2016, Advance Article
DOI: 10.1039/C5QO00417A, Research Article
An intramolecular copper-catalyzed direct C(sp2)–H activation/C(sp2)–N bond formation reaction has been developed for the synthesis of pyrrolo[3,2-c]quinolinone derivatives under an oxygen atmosphere. This approach presents an alternative route to the tricyclic core of martinellic acid or martinelline.
 
Org. Chem. Front., 2016, Advance Article
DOI: 10.1039/C5QO00346F, Research Article
From themed collection 2015 Emerging Investigators by OCF
Dearomative cycloadditions of imino esters derived from alanine with 3-nitroindoles form exo′-pyrroloindolines in good yields with high diastereo- and enantioselectivities.
 
Org. Chem. Front., 2016, Advance Article
DOI: 10.1039/C5QO00372E, Research Article
From themed collection 2015 Emerging Investigators by OCF
The novel NHC-catalyzed dehydrogenative coupling of enals is described to generate a wide range of monobactams.
 
Org. Chem. Front., 2016, Advance Article
DOI: 10.1039/C5QO00354G, Research Article
From themed collection 2015 Emerging Investigators by OCF
The Au-catalyzed tandem reaction provided simple and efficient access to spiro-dipyrroloquinolines and incargranine B aglycone and (±)-seneciobipyrrolidine (I).
 
Org. Chem. Front., 2016, Advance Article
DOI: 10.1039/C5QO00315F, Research Article
The intramolecular aza-(4 + 3) cycloaddition reactions of in situ generated aza-oxyallylic cations and furans have been reported for the construction of medium sized hydroxamate macrocycles.
 
Org. Chem. Front., 2016, Advance Article
DOI: 10.1039/C5QO00361J, Research Article
From themed collection 2015 Emerging Investigators by OCF
A novel iodine(III)-mediated synthesis of substituted phenanthrenes from ortho-vinylated biaryl derivatives through 6-endo-trig selective oxidative intramolecular arene–alkene coupling is reported.
 

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