Journal cover: Organic Chemistry Frontiers

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Org. Chem. Front., 2014, Advance Article
DOI: 10.1039/C4QO00196F, Research Article
Using an oxidizing directing group, a mild RuII-catalyzed direct coupling of N-phenoxypivalamide with internal alkynes was developed, generating the benzofurans in moderate to high yields.
 
Org. Chem. Front., 2014, Accepted Manuscript
DOI: 10.1039/C4QO00214H, Research Article
Density functional theory calculations were carried out to study the Pd-catalysed oxidation reactions of alcohols using phenyl chloride as oxidant. Our calculations supported that the mechanism mainly involves oxidative addition,...
 
Org. Chem. Front., 2014, Advance Article
DOI: 10.1039/C4QO00231H, Review Article
Metal-mediated organic reactions have become one of the great frontiers of organic synthesis.
 
Org. Chem. Front., 2014, Advance Article
DOI: 10.1039/C4QO00218K, Research Article
Alkenyl nitriles can be easily accessed by Pd(II)-catalyzed reaction of allyl arenes with tert-butyl nitrite as both the nitrogen source and oxidant and N-hydroxyphthalimide as the co-catalyst.
 
Org. Chem. Front., 2014, Advance Article
DOI: 10.1039/C4QO00206G, Research Article
Iron-catalyzed regio- and stereoselective 1,4-hydroborations of 1,3-dienes produce secondary benzylic (Z)-allylboronates.
 
Hisanori Itoh, Hironori Maeda, Shinya Yamada, Yoji Hori, Takashi Mino and Masami Sakamoto
Org. Chem. Front., 2014, Advance Article
DOI: 10.1039/C4QO00222A, Research Article
We developed a highly reactive catalytic ring-closing ene reaction with chiral aluminum complexes. Kinetic resolutions of citronellal successfully afforded 68% ee of diastereoselective isopulegol and 62% ee of citronellal at 47% conversion with the BINOL-Al catalyst. L-Menthol was synthesized from citral with kinetic resolutions.
 
Org. Chem. Front., 2014, Advance Article
DOI: 10.1039/C4QO00210E, Research Article
The first example of the application of a chiral DMAP catalyst for allylic substitution of MBH carbonates.
 
Org. Chem. Front., 2014, Advance Article
DOI: 10.1039/C4QO00157E, Research Article
Copper(I)-catalyzed enantioselective hydroboration of 3-aryl substituted cyclopropene-3-carboxylate is described, providing chiral cyclopropylboronates with excellent enantioselectivities (89–95% ee) in moderate to high yields (55–86%).
 
Jian-Bo Zhu, Hao Chen, Saihu Liao, Yu-Xue Li and Yong Tang
Org. Chem. Front., 2014, Advance Article
DOI: 10.1039/C4QO00232F, Research Article
The first phosphine-catalyzed cyclopropanation reaction via covalent ylide catalysis has been realized with high efficiency in the presence of sidearm-assisted phosphine catalysts.
 
Yi-Chao Huang, Cheng Cao, Xiang-Long Tan, Xiaoyu Li and Lei Liu
Org. Chem. Front., 2014, Advance Article
DOI: 10.1039/C4QO00217B, Research Article
A p-nitrobenzyloxycarbonyl/bis-Boc strategy was developed for efficient synthesis of versatile PNA–peptide conjugates.
 
Thanh Binh Nguyen, Ludmila ERMOLENKO, Mathilde Corbin and Ali ALMOURABIT
Org. Chem. Front., 2014, Accepted Manuscript
DOI: 10.1039/C4QO00221K, Research Article
Fe/S clusters generated in situ from simple iron salts and sulfur S8 were found to be highly efficient to catalyze the decarboxylative redox condensation of arylacetic acids with nitro arenes...
 
Org. Chem. Front., 2014, Accepted Manuscript
DOI: 10.1039/C4QO00205A, Research Article
This paper describes the direct C-H bond cyanation of 2-phenylpyridines employing N,N-dimethylformamide (DMF) as both reagent and solvent. DMF provides both of the C and N unit in the generated...
 
Wen-Jing Xuan, Candice Botuha, Bernold Hasenknopf and Serge Thorimbert
Org. Chem. Front., 2014, Advance Article
DOI: 10.1039/C4QO00193A, Research Article
Organic soluble TBA5K[α1Hf(H2O)4P2W17O61] (POM/Hf) catalyzes the addition of pronucleophiles (silylenolethers, diketones, ketoesters, allylsilane) to unactivated hemiaminals.
 
Org. Chem. Front., 2014, Advance Article
DOI: 10.1039/C4QO00172A, Research Article
Oxidant controlled selective C–H bond mono-alkenylation and di-alkenylation of biphenylthioethers to synthesize sulfoxide-olefin ligands with thioether as the directing group.
 
Org. Chem. Front., 2014, Accepted Manuscript
DOI: 10.1039/C4QO00233D, Research Article
A robust catalyst derived from NiCl2•(DME) and acenaphthoimidazolium chloride exhibited high activity towards challenging amination of bulky and heterocyclic aryl tosylates with secondary amines under mild reaction conditions at 2...
 
Org. Chem. Front., 2014, Advance Article
DOI: 10.1039/C4QO00185K, Research Article
A versatile fluorescent probe NPS that displayed high selectivity for Hg2+ in aqueous solution and living cells has been developed.
 
Org. Chem. Front., 2014, Accepted Manuscript
DOI: 10.1039/C4QO00208C, Review Article
While one-carbon central chirality of organic molecules has been recognized and extensively studied for more than a century, far less attention has been paid to three-carbon axial chirality of allenes,...
 
Xiaoxi Zhou, Chunhong Zhang, Yumei Lin, Xumin He, Yan Zhang, Jianbo Wang and Haiping Xia
Org. Chem. Front., 2014, Advance Article
DOI: 10.1039/C4QO00152D, Research Article
1,2-Migration in the reactions of ruthenium vinyl carbene with propargyl alcohols has been investigated, the migratory preference is H > Ph > CH3.
 
Org. Chem. Front., 2014, Advance Article
DOI: 10.1039/C4QO00202D, Research Article
From themed collection In Celebration of Max Malacria’s 65th Birthday
A metal-free reductive procedure for decyanation of malononitriles and cyanoacetates, using photoactivated organic electron donors, is described.
 
Org. Chem. Front., 2014, Advance Article
DOI: 10.1039/C4QO00198B, Research Article
The Sonogashira reaction under non-basic conditions.
 
Org. Chem. Front., 2014, Advance Article
DOI: 10.1039/C4QO00209A, Research Article
1-Amino-isoquinoline-N-oxides are generated under mild conditions in good yields through a silver(I) and copper(I) catalyzed reaction of 2-alkynylbenzaldoxime with secondary amines.
 
Org. Chem. Front., 2014, Advance Article
DOI: 10.1039/C4QO00180J, Research Article
From themed collection In Celebration of Max Malacria’s 65th Birthday
Enantioselective synthesis of a key intermediate to (−)-huperzine A by Pd-catalyzed tandem allylic alkylation using a novel monodentate phosphoramidite ligand.
 
Org. Chem. Front., 2014, Advance Article
DOI: 10.1039/C4QO00179F, Research Article
From themed collection In Celebration of Max Malacria’s 65th Birthday
Palladium-catalyzed amino and oxyacetoxylation have been developed to furnish 1,4-benzodiazepinones and 1,4-benzoxazepinones through the diheterofunctionalization of alkenes.
 
Zhenbo Mo, Zhenwu Ouyang, Lei Wang, Kathlyn L. Fillman, Michael L. Neidig and Liang Deng
Org. Chem. Front., 2014, Advance Article
DOI: 10.1039/C4QO00175C, Research Article
Monodentate aminocarbene ligands, both NHC and cAAC, are capable of stabilizing low-coordinate iron(I) compounds.
 
Org. Chem. Front., 2014, Advance Article
DOI: 10.1039/C4QO00189C, Highlight
New members in the family of organophosphorus compounds: convenient synthesis and reactivity of the 2-phosphaethynolate anion are highlighted.
 

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