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Journal cover: Organic Chemistry Frontiers

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Impact Factor 4.693 12 Issues per Year Free access available
 
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Susan M Stevenson, Eric T Newcomb and Eric Matthew Ferreira
Org. Chem. Front., 2016, Accepted Manuscript
DOI: 10.1039/C6QO00224B, Research Article
From themed collection Celebrating the 75th Birthday of Professor Barry Trost
A full account of our investigation of C–C bond migration in the cycloisomerization of oxygen-tethered 1,6-enynes is described. Under Pt(II) and/or Ir(I) catalysis, cyclic and acylic alkyl groups were found...
 
Org. Chem. Front., 2016, Advance Article
DOI: 10.1039/C6QO00178E, Research Article
Pd-catalyzed difluoroallylation of unactivated C(sp2)–H bonds with readily available Rf-Br reagents is described.
 
Toru Amaya, Izumi Kurata and Toshikazu Hirao
Org. Chem. Front., 2016, Advance Article
DOI: 10.1039/C6QO00107F, Research Article
From themed collection Celebrating the 75th Birthday of Professor Barry Trost
The synthesis of 3-aryl-3-hydroxy-2-oxindoles, which are a structural motif found in various natural products and pharmaceutically active compounds, was conducted via reductive coupling of (2-aminophenyl)(aryl)methanone derivatives and CO2 as a key step. The conditions employing Mg with chlorotrimethylsilane in DMA are the best for the reductive coupling. The reductive coupling and acid-catalyzed lactam formation can be performed in a one-pot reaction to give the oxindoles.
 
Org. Chem. Front., 2016, Accepted Manuscript
DOI: 10.1039/C6QO00204H, Research Article
From themed collection Celebrating the 75th Birthday of Professor Barry Trost
Through-space conjugation is conducive to efficient multidimensional exciton diffusion and charge transport in optoelectronic functional materials. Herein, a series of tetraphenylethene derivatives with through-space conjugation formed between benzene and various...
 
Org. Chem. Front., 2016, Accepted Manuscript
DOI: 10.1039/C6QO00208K, Research Article
From themed collection Celebrating the 75th Birthday of Professor Barry Trost
The diastereo- and enantioselective synthesis of cyclohexanone-fused spirospyrazolones containing four consecutive chiral centers has been successfully developed through an asymmetric Michael/Michael/aldol cascade reaction catalyzed by the combination of the bifunctional...
 
Io Sato, Hirotsugu Suzuki, Yasuhiro Yamashita and Shu Kobayashi
Org. Chem. Front., 2016, Accepted Manuscript
DOI: 10.1039/C6QO00242K, Research Article
From themed collection Celebrating the 75th Birthday of Professor Barry Trost
In the presence of catalytic amounts of potassium hexamethyldisilazide (KHMDS) and a chiral macrocyclic crown ether, asymmetric 1,4-addition reactions of simple esters with α,β-unsaturated amides proceeded to afford the desired...
 
Pierrick Ondet, Luisa Lempenauer, Elisabet Duñach and Gilles Lemière
Org. Chem. Front., 2016, Advance Article
DOI: 10.1039/C6QO00212A, Research Article
A series of complex polycyclic ethers have been synthesised under very mild conditions using a low catalyst loading of bismuth(III) triflate.
 
Org. Chem. Front., 2016, Accepted Manuscript
DOI: 10.1039/C6QO00227G, Research Article
From themed collection Celebrating the 75th Birthday of Professor Barry Trost
A novel type of binaphthyl-based phosphoramidite-thioether ligands have been developed and successfully applied to Pd-catalysed asymmetric C-3 allylic alkylation of indoles, giving the desired products with up to 99% yield...
 
Hideki Abe, Takuma Hikichi, Kosuke Emori, Toyoharu Kobayashi and Hisanaka Ito
Org. Chem. Front., 2016, Accepted Manuscript
DOI: 10.1039/C6QO00213G, Research Article
From themed collection Celebrating the 75th Birthday of Professor Barry Trost
The asymmetric total synthesis of catunaregin isolated from the Chinese mangrove is described. The synthesis involves an asymmetric syn-selective aldol reaction and the successive ketalization of a furan diol derivative...
 
Org. Chem. Front., 2016, Advance Article
DOI: 10.1039/C6QO00169F, Research Article
A zinc-catalyzed oxidative reaction of ynamides with phenols and thiophenols under mild reaction conditions has been developed, which provides various α-aryloxy amides and α-arylthio amides in moderate to good yields, respectively. Importantly, high chemoselectivity is achieved by such a non-noble metal-catalyzed alkyne oxidation.
 
Org. Chem. Front., 2016, Advance Article
DOI: 10.1039/C6QO00267F, Research Article
A photoinduced radical cyclization of benzene-tethered 1,7-enynes with Togni reagent in the presence of sodium iodide is developed. This transformation works well without any metals or photo-redox catalysts at room temperature.
 
Org. Chem. Front., 2016, Advance Article
DOI: 10.1039/C6QO00153J, Review Article
Recent advances in photoinduced trifluoromethylation and difluoroalkylation under photocatalysis are summarized. Most of the photoredox reactions proceed efficiently under mild conditions with simple operation. Various fluorinated reagents are developed and applied in different transformations.
 
Chung-kay Edwin Law and István T. Horváth
Org. Chem. Front., 2016, Advance Article
DOI: 10.1039/C6QO00115G, Review Article
From themed collection Celebrating the 75th Birthday of Professor Barry Trost
The synthesis, some of the properties and the applications of fluorous phosphines in biphasic, organometallic and organo-catalysis were reviewed.
 
Org. Chem. Front., 2016, Accepted Manuscript
DOI: 10.1039/C6QO00210B, Review Article
From themed collection Celebrating the 75th Birthday of Professor Barry Trost
With the advent of directed evolution of stereoselective enzymes almost 20 years ago and the rapid development of this exciting area of research, the traditional limitations of biocatalysts in organic...
 
Org. Chem. Front., 2016, Advance Article
DOI: 10.1039/C6QO00156D, Review Article
Recent advances in copper-mediated (both stoichiometric and catalytic) chelation-assisted functionalization of unactivated C–H bonds are reviewed.
 
Org. Chem. Front., 2016, Advance Article
DOI: 10.1039/C6QO00099A, Research Article
A cobalt-promoted coupling reaction of triethoxysilanes, sulfur dioxide, and electrophiles is developed. Different electrophilic partners including alkyl bromides, iodonium salts, and electron-poor (hetero)aryl chlorides work well under the standard conditions.
 
Kohei Watanabe, Takashi Mino, Tatsuya Ikematsu, Chikako Hatta, Yasushi Yoshida and Masami Sakamoto
Org. Chem. Front., 2016, Advance Article
DOI: 10.1039/C6QO00112B, Research Article
From themed collection Celebrating the 75th Birthday of Professor Barry Trost
The annulation of 1-cinnamyloxy-2-ethynylbenzene derivatives using a hydrazone–palladium catalyst system proceeded smoothly and gave the corresponding 2-substituted-3-cinnamylbenzofurans in good-to-excellent yields.
 
Guanghui Zhang, Hong Yi, Jie Xin, Yi Deng, Ruopeng Bai, Zhiliang Huang, Jeffrey T. Miller, A. Jeremy Kropf, Emilio E. Bunel, Xiaotian Qi, Yu Lan and Aiwen Lei
Org. Chem. Front., 2016, Advance Article
DOI: 10.1039/C6QO00201C, Research Article
Ate-complex [Cu(OtBu)2]Na was found to be able to cleave C–H bond of benzothiazole (ArH) producing [ArCuI(OtBu)]Na with a rate constant of 3.2 × 10−2 mol−1 L s−1 at −50 °C and with an activation enthalpy of 0.73 kcal mol−1 at room temperature.
 
Org. Chem. Front., 2016, Advance Article
DOI: 10.1039/C6QO00119J, Research Article
From themed collection Celebrating the 75th Birthday of Professor Barry Trost
A versatile cascade route to cyclic imides via direct functionalization of the β-alkenyl C–H bond of alkenoic acids was developed.
 
Org. Chem. Front., 2016, Advance Article
DOI: 10.1039/C6QO00103C, Review Article
Recent developments in the photochemical carbon–carbon and carbon–heteroatom bond formation via photoinduced Ar–X bond dissociation are summarized. Under ultraviolet irradiation, the reactions of aryl halides with reactive partners proceed smoothly under mild conditions. In some cases, the transformations proceed without any metals or photo-redox catalysts.
 
Org. Chem. Front., 2016, Advance Article
DOI: 10.1039/C6QO00197A, Research Article
From themed collection Celebrating the 75th Birthday of Professor Barry Trost
A supramolecular polyrotaxane constructed by pillar[5]arene-based pseudo[2]rotaxanes via the incorporation of metal–ligand coordination could further self-assemble to form a stimuli-responsive supramolecular gel at high concentration.
 
Tatiana Besset, Philippe Jubault, Xavier Pannecoucke and Thomas Poisson
Org. Chem. Front., 2016, Advance Article
DOI: 10.1039/C6QO00164E, Highlight
The OCF3 group is of high interest in the quest for new drugs and agrochemicals, thanks to its atypical features. This Highlight article depicted the recent and impressive advances toward the synthesis of OCF3-containing molecules.
 
Org. Chem. Front., 2016, Advance Article
DOI: 10.1039/C6QO00198J, Research Article
A series of unsymmetrical palladacycles have been synthesised and evaluated as catalysts in aldol and vinyl epoxide coupling chemistry.
 
Wenlei Zhai, Brette M. Chapin, Akina Yoshizawa, Hui-Chen Wang, Stephen A. Hodge, Tony D. James, Eric V. Anslyn and John S. Fossey
Org. Chem. Front., 2016, Advance Article
DOI: 10.1039/C6QO00171H, Research Article
A series of boronic acid-containing saccharide receptors was synthesised via copper catalysed azide–alkyne cycloaddition (CuAAC) reactions.
 
Org. Chem. Front., 2016, Advance Article
DOI: 10.1039/C6QO00116E, Research Article
A novel approach has been reported for the preparation of biaryl sultams using visible-light-promoted denitrogenative cyclization of 1,2,3,4-benzothiatriazine-1,1-dioxides.
 

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