Journal cover: Organic Chemistry Frontiers

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Org. Chem. Front., 2015, Advance Article
DOI: 10.1039/C4QO00319E, Research Article
From themed collection Celebrating the 80th Birthday of Professor Ei-ichi Negishi
Ru-catalyzed dehydrogenative amide synthesis from aldehydes and amines was achieved, based on the idea of using a hemiaminal intermediate to generate the active Ru-hydride species.
 
Zining Li, Qian Geng, Zhe Lv, Beau P. Pritchett, Katsuaki Baba, Yoshitaka Numajiri, Brian M. Stoltz and Guangxin Liang
Org. Chem. Front., 2015, Advance Article
DOI: 10.1039/C4QO00312H, Research Article
Selective syntheses of alkaloids bearing distinct core structures were enabled by chemically programmed polycyclizations using water as a switch.
 
Org. Chem. Front., 2015, Advance Article
DOI: 10.1039/C4QO00301B, Research Article
Palladium-catalyzed cyanation of aryldiazonium tetrafluoroborate using acetonitrile as a non-metallic cyanide source was achieved in the presence of Ag2O under ambient air, eliminating the involvement of highly toxic CuCN used in the traditional Sandmeyer reaction, in which the CN group comes from metallic cyanides.
 
N. Kodiah Beyeh, Arto Valkonen, Sandip Bhowmik, Fangfang Pan and Kari Rissanen
Org. Chem. Front., 2015, Accepted Manuscript
DOI: 10.1039/C4QO00326H, Research Article
N-Cyclohexyl ammonium resorcinarene halides, stabilized by an intricate array of hydrogen bonds into a cavitand-like assembly, forms multivalent halogen bonded deep cavity cavitands with perfluoroiodobenzenes. From macromolar to infinite concentration...
 
Org. Chem. Front., 2015, Accepted Manuscript
DOI: 10.1039/C4QO00316K, Research Article
From themed collection Celebrating the 80th Birthday of Professor Ei-ichi Negishi
We have employed 4-alkenyl-5H-1,2,3-oxathiazole 2,2-dioxides as useful reagents able to generate in situ an electron-rich diene intermediate that has the potential to undergo [4+2] cycloaddition with a,b-unsaturated aldehydes through the...
 
Ren-Rong Liu, Zheng-Yi Cai, Chuan-Jun Lu, Shi-Chun Ye, Bin Xiang, Jianrong Gao and Yi-Xia Jia
Org. Chem. Front., 2015, Advance Article
DOI: 10.1039/C4QO00336E, Research Article
Cu-catalyzed cyclization of 2-(2-enynyl)pyridines with various nucleophiles was developed, providing efficient access to indolizine derivatives.
 
Org. Chem. Front., 2015, Advance Article
DOI: 10.1039/C4QO00261J, Research Article
A gold-catalyzed asymmetric intermolecular [3 + 2]-cycloaddition of γ-1-ethoxyethoxy-propiolate and aldehydes by using the chiral ligand 5a or 5b is developed, which provides facile access to highly substituted 2,5-dihydrofurans in up to 84% yield with up to 97% ee.
 
Org. Chem. Front., 2015, Advance Article
DOI: 10.1039/C4QO00314D, Research Article
Direct oxidative C(sp3)–H functionalization of acetonitrile and alkanes with α,α-diaryl allylic alcohols has been developed.
 
Buddha B. Khatri, Svitlana Kulyk and Scott McN. Sieburth
Org. Chem. Front., 2015, Advance Article
DOI: 10.1039/C5QO90005K, Correction
 
Org. Chem. Front., 2015, Accepted Manuscript
DOI: 10.1039/C4QO00321G, Research Article
N,N,P-Pincer-nickel-complex-catalyzed cross-coupling of aryltrimethylammonium triflates with aryl- or heteroaryl-zinc reagents was investigated. The reaction suits for a broad scope of substrates, exhibits good functional group compatibility and can be performed...
 
Org. Chem. Front., 2015, Advance Article
DOI: 10.1039/C4QO00323C, Research Article
From themed collection Celebrating the 80th Birthday of Professor Ei-ichi Negishi
Catalytic amounts of the base catalyst DABCO in cooperation with a proton source afford the [4 + 2] cycloadducts of isatins with but-3-yn-2-one in moderate to good yields. Moreover, related plausible mechanisms have been proposed in detail based on control and deuterium labeling experiments.
 
Org. Chem. Front., 2015, Advance Article
DOI: 10.1039/C4QO00333K, Research Article
From themed collection Celebrating the 80th Birthday of Professor Ei-ichi Negishi
Regioselective H/D exchange reaction of functional groups on heterocycles proceeded via a transition metal-free reductive cyclization of sulfanyl 1,6-diynes using sodium borodeuteride/ethanol-D1.
 
Jian Zhao, Kazuaki Oniwa, Ashraful Islam, Chuanjiang Qin, Naoki Asao, Liyuan Han, Yoshinori Yamamoto and Tienan Jin
Org. Chem. Front., 2015, Accepted Manuscript
DOI: 10.1039/C4QO00285G, Research Article
From themed collection Celebrating the 80th Birthday of Professor Ei-ichi Negishi
A new series of donor-π-acceptor organic K-dyes based on thieno[2,3,a]carbazole moiety as a new electron donor, trithiophene as a π-linker and cyanoacrylic acid as an electron acceptor were designed and...
 
Tong-Hao Zhu, Tian-Qi Wei, Shun-Yi Wang and Shun-Jun Ji
Org. Chem. Front., 2015, Accepted Manuscript
DOI: 10.1039/C4QO00289J, Research Article
A NIS/CHP mediated [4+1]-cycloaddition of isocyanides with in situ generated 1,2-diaza-1,3-dienes from hydrazones under metal-free conditions has been developed. This protocol provides a new, atom efficient and step efficient way...
 
Org. Chem. Front., 2015, Advance Article
DOI: 10.1039/C4QO00294F, Review Article
This review summarizes recent progress in catalytic asymmetric construction of 1,2,3,4-tetrahydroisoquinolines and 3,4-dihydroisoquinolines, among the most important “privileged scaffolds”.
 

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