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Physical Chemistry Chemical Physics

High quality research in physical chemistry, chemical physics and biophysical chemistry.
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Physical Chemistry Chemical Physics,
21 February 2011 , Issue 7,
Page 2425 to 2980
Phys. Chem. Chem. Phys., 2011, 13, 2447-2448
DOI: 10.1039/C1CP90005F, Editorial
From themed collection Controlled nanostructures for applications in catalysis
Assembly of solid catalysts from pre-fabricated components, control of structures, sizes, and localization of nanoparticles on support materials, and tailoring of pore structures in solid catalysts have made such great progress that a special issue devoted to these topics seemed called for to provide a survey of this field.
 
Ilkeun Lee, Manuel A. Albiter, Qiao Zhang, Jianping Ge, Yadong Yin and Francisco Zaera
Phys. Chem. Chem. Phys., 2011, 13, 2449-2456
DOI: 10.1039/C0CP01688H, Perspective
From themed collection Controlled nanostructures for applications in catalysis
Novel nanoarchitectures are being developed using colloidal and other self-assembly synthetic methods for the design of heterogeneous catalysts with heightened selectivity and stability.
 
Phys. Chem. Chem. Phys., 2011, 13, 2457-2487
DOI: 10.1039/C0CP02680H, Perspective
From themed collection Controlled nanostructures for applications in catalysis
The use of pre-prepared colloidal metal nanoparticles with tuned size, shape and composition as components of designed catalysts opens up a new field in catalysis.
 
Phys. Chem. Chem. Phys., 2011, 13, 2488-2491
DOI: 10.1039/C0CP01309A, Communication
From themed collection Controlled nanostructures for applications in catalysis
Well-dispersed noble metal nanoparticles can be synthesized, and further stabilized under high treatment temperature, by the confinement effect of ordered mesoporous alumina.
 
Richard T. Mayes, Pasquale F. Fulvio, Zhen Ma and Sheng Dai
Phys. Chem. Chem. Phys., 2011, 13, 2492-2494
DOI: 10.1039/C0CP01861A, Communication
From themed collection Controlled nanostructures for applications in catalysis
A soft-templated mesoporous carbon has been phosphorylated at room temperature to produce surface acidic sites active toward isopropanol dehydration.
 
Phys. Chem. Chem. Phys., 2011, 13, 2495-2503
DOI: 10.1039/C0CP01807D, Paper
From themed collection Controlled nanostructures for applications in catalysis
Ordered mesoporous carbon supported nanosized calcium oxides were synthesized, showing promising CO2 capture properties through both physi- and chemisorption.
 
Phys. Chem. Chem. Phys., 2011, 13, 2504-2511
DOI: 10.1039/C0CP01828G, Paper
From themed collection Controlled nanostructures for applications in catalysis
The microenvironment of the nanocages had a big influence on the catalytic activity and enantioselectivity for the asymmetric catalysis.
 
Youngjin Jang, Jooyoung Chung, Seyoung Kim, Samuel Woojoo Jun, Byung Hyo Kim, Dong Won Lee, B. Moon Kim and Taeghwan Hyeon
Phys. Chem. Chem. Phys., 2011, 13, 2512-2516
DOI: 10.1039/C0CP01680B, Paper
From themed collection Controlled nanostructures for applications in catalysis
Pd–Fe3O4 heterodimer nanocrystals, synthesized by controlled one-pot thermolysis, exhibit good catalytic activities and recyclability for various Suzuki coupling reactions.
 
Matthew B. Boucher, Simone Goergen, Nan Yi and Maria Flytzani-Stephanopoulos
Phys. Chem. Chem. Phys., 2011, 13, 2517-2527
DOI: 10.1039/C0CP02009E, Paper
From themed collection Controlled nanostructures for applications in catalysis
Structure-controlled metal oxide nanoshapes were used to bind and disperse highly active gold species for the WGS and SRM reactions.
 
Albert F. Carley, David J. Morgan, Nianxue Song, M. Wyn Roberts, Stuart H. Taylor, Jonathan K. Bartley, David J. Willock, Kara L. Howard and Graham J. Hutchings
Phys. Chem. Chem. Phys., 2011, 13, 2528-2538
DOI: 10.1039/C0CP01852J, Paper
From themed collection Controlled nanostructures for applications in catalysis
The unexpected observation of CO bond cleavage over Au/Fe2O3 catalysts is investigated using TAP reactor studies, XPS and DFT calculations.
 
Francesca Bleken, Wegard Skistad, Katia Barbera, Marina Kustova, Silvia Bordiga, Pablo Beato, Karl Petter Lillerud, Stian Svelle and Unni Olsbye
Phys. Chem. Chem. Phys., 2011, 13, 2539-2549
DOI: 10.1039/C0CP01982H, Paper
From themed collection Controlled nanostructures for applications in catalysis
3D 10-ring zeolites with varying channel intersections exhibit similar product distribution but different catalyst life-time and coke-selectivity in MTH.
 
Aihua Zhang, Shouli Sun, Zachary J. A. Komon, Neil Osterwalder, Sagar Gadewar, Peter Stoimenov, Daniel J. Auerbach, Galen D. Stucky and Eric W. McFarland
Phys. Chem. Chem. Phys., 2011, 13, 2550-2555
DOI: 10.1039/C0CP01985B, Paper
From themed collection Controlled nanostructures for applications in catalysis
Increasing the ratio of Si/Al and incorporation of Co into the catalyst framework improves the yield of ethylene and propylene from the reaction of methyl bromide.
 
James Russell Renzas, Wenyu Huang, Yawen Zhang, Michael E. Grass, Dat Tien Hoang, Selim Alayoglu, Derek R. Butcher, Franklin (Feng) Tao, Zhi Liu and Gabor A. Somorjai
Phys. Chem. Chem. Phys., 2011, 13, 2556-2562
DOI: 10.1039/C0CP01858A, Paper
From themed collection Controlled nanostructures for applications in catalysis
Rh1−x-shell/Pdx-core nanoparticle catalysts in CO oxidation were found to exhibit enhanced catalytic activity versus monometallic catalysts in oxygen-rich conditions.
 
Toshiyuki Yokoi, Junya Sakuma, Kazuhiko Maeda, Kazunari Domen, Takashi Tatsumi and Junko N. Kondo
Phys. Chem. Chem. Phys., 2011, 13, 2563-2570
DOI: 10.1039/C0CP02141E, Paper
From themed collection Controlled nanostructures for applications in catalysis
The colloidal array of NaTaO3 nanoparticles 20 nm in size has been successfully prepared by hydrothermal synthesis through the reaction of NaOH solution and Ta2O5 in a three-dimensional mesoporous carbon as the template.
 
J. Chris Bauer, David Mullins, Meijun Li, Zili Wu, E. Andrew Payzant, Steven H. Overbury and Sheng Dai
Phys. Chem. Chem. Phys., 2011, 13, 2571-2581
DOI: 10.1039/C0CP01859G, Paper
From themed collection Controlled nanostructures for applications in catalysis
We report the synthesis of silica-supported AuCu nanoparticles through the conversion of supported Au nanoparticles with a solution-based methodology for catalysis.
 
Zhi Li, Cristian V. Ciobanu, Juncheng Hu, Juan-Pedro Palomares-Báez, José-Luis Rodríguez-López and Ryan Richards
Phys. Chem. Chem. Phys., 2011, 13, 2582-2589
DOI: 10.1039/C0CP01820A, Paper
From themed collection Controlled nanostructures for applications in catalysis
Gold nanoparticles on MgO nanosheets (TEM image, left) and simplified structural model showing charge transfer at the Au/MgO(111)–O interface (right).
 
William O. Oduro, Nick Cailuo, Kai Man K. Yu, Hongwei Yang and Shik Chi Tsang
Phys. Chem. Chem. Phys., 2011, 13, 2590-2602
DOI: 10.1039/C0CP01832E, Paper
From themed collection Controlled nanostructures for applications in catalysis
A model showing transition metal atoms decorating on corner sites of Pt nanocrystal can exert a strong geometric and electronic influence on catalytic pathways in hydrogenation of cinnamaldehyde.
 
Phys. Chem. Chem. Phys., 2011, 13, 2603-2612
DOI: 10.1039/C0CP01996H, Paper
From themed collection Controlled nanostructures for applications in catalysis
Dispersion corrected DFT explains the catalytic behavior of acid sites in 8MR and 12MR MOR channels in methanol/DME carbonylation.
 
Phys. Chem. Chem. Phys., 2011, 13, 2613-2626
DOI: 10.1039/C0CP01971B, Perspective
Electrostatic interactions between ions are exaggerated in non-polarizable MD simulations by a factor of about 2. A simple consistent solution is presented.
 
Radovan Bast, Ulf Ekström, Bin Gao, Trygve Helgaker, Kenneth Ruud and Andreas J. Thorvaldsen
Phys. Chem. Chem. Phys., 2011, 13, 2627-2651
DOI: 10.1039/C0CP01647K, Perspective
A complete computational approach for calculating molecular properties involving any element in the periodic table is presented.
 
Shanthi Murali, Daniel R. Dreyer, Patricia Valle-Vigón, Meryl D. Stoller, Yanwu Zhu, Cornelio Morales, Antonio B. Fuertes, Christopher W. Bielawski and Rodney S. Ruoff
Phys. Chem. Chem. Phys., 2011, 13, 2652-2655
DOI: 10.1039/C0CP02557G, Communication
The performance of mesoporous carbon capsules as electrode materials in electrochemical double layer capacitors (EDLCs) was evaluated in the presence of a variety of electrolytes, including room temperature ionic liquids (ILs).
 
Beibei Ma, Liduo Wang, Haopeng Dong, Rui Gao, Yi Geng, Yifeng Zhu and Yong Qiu
Phys. Chem. Chem. Phys., 2011, 13, 2656-2658
DOI: 10.1039/C0CP02415E, Communication
The optical and electrical properties of PbS QDs synthesized by a photocatalysis method using the photocatalytic activity of TiO2 were studied.
 
Phys. Chem. Chem. Phys., 2011, 13, 2659-2662
DOI: 10.1039/C0CP02209H, Communication
The NH edge is an active site of the nitrided graphite and facilitates easy transfer of an electron into the adsorbed O2.
 
Phys. Chem. Chem. Phys., 2011, 13, 2663-2666
DOI: 10.1039/C0CP01870H, Communication
Monte Carlo simulations of the coarsening of oxide particle containing liquid lithium electrolytes explains the conductivity transients for typical soggy sand electrolytes as well as the evolution towards a stationary conductivity.
 
Lianqin Wang, Hui Meng, Pei Kang Shen, Claudio Bianchini, Francesco Vizza and Zidong Wei
Phys. Chem. Chem. Phys., 2011, 13, 2667-2673
DOI: 10.1039/C0CP01913E, Paper
This in situ FTIR spectroelectrochemical study shows that the products of ethylene glycol oxidation on a Pd electrode are influenced by pH.
 

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