Issue 29, 2013

Half-metallic perovskite superlattices with colossal thermoelectric figure of merit

Abstract

Nowadays heavy experimental efforts are focussed on doped oxide thermoelectrics to increase the thermopower and thermoelectric performance. We propose a high thermoelectric figure of merit for half-metallic SrTi1−xCoxO3 (x = 0, 0.125, 0.25, 0.375, and 0.5) in a superlattice with SrTiO3, which is stable at high temperatures and in an oxygen environment. The maximal value of Z hardly depends on the doping, while the temperature at which the maximum occurs increases with the Co concentration. The easy tunability from being an insulator to a half-metal under substitutional doping combined with the colossal figure of merit opens up great potential in the emerging field of spin-caloritronics.

Graphical abstract: Half-metallic perovskite superlattices with colossal thermoelectric figure of merit

Article information

Article type
Paper
Submitted
03 Apr 2013
Accepted
08 May 2013
First published
09 May 2013

J. Mater. Chem. A, 2013,1, 8406-8410

Half-metallic perovskite superlattices with colossal thermoelectric figure of merit

M. U. Kahaly, K. Ozdogan and U. Schwingenschlögl, J. Mater. Chem. A, 2013, 1, 8406 DOI: 10.1039/C3TA11346A

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