Heterometallic 3d–4f polyoxometalates still remain as an almost unexplored class of polyoxoanions despite showing great potential in fields such as molecular magnetism. This Frontier reviews some of their synthetic, structural and magnetic features and gives a personal view on future research in this area.
S. Reinoso, Dalton Trans., 2011, 40, 6610 DOI: 10.1039/C1DT10174A
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