A series of Fe(III) salts and organic solvents have been screened to develop novel non-aqueous catalysts for the conversion of H2S to sulfur. FeCl3/95% N-methylpyrrolidinone/5% H2O was found to be a most efficient non-aqueous system. The process chemistry, the proposed mechanism of catalytic oxidation of H2S, and the electrochemistry are discussed.
G. Hua, Q. Zhang, D. McManus, A. M. Z. Slawin and J. D. Woollins, Dalton Trans., 2006, 1147 DOI: 10.1039/B513384J
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