In non-catalytic direct conversion of methane to acetylene by using direct current pulse discharge under conditions of ambient temperature and atmospheric pressure, the selectivity of acetylene from methane was >95% at methane conversion ranging from 16 to 52%; coexisting oxygen was very effective in removing deposited carbon and stabilized the state of discharge.
S. Kado, Y. Sekine and K. Fujimoto, Chem. Commun., 1999, 2485 DOI: 10.1039/A906914C
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