An X-ray crystallographic structure determination of the nitrate salt of the gadolinium imBT cryptate shows coordination of two water molecules; NMRD relaxometry of this cryptate reveals a relaxivity of 5.8 mM–1 s–1 (at 10 MHz, 298 K and pH 6), which is pH sensitive over the range 4–9.
S. W. Annie Bligh, M. G. B. Drew, N. Martin, B. Maubert and J. Nelson, J. Chem. Soc., Dalton Trans., 1998, 3711 DOI: 10.1039/A805859H
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