This article presents the progress made in probing femtosecond transition–state dynamics of elementary reactions. Experiments demonstrating the dynamics in systems characterized by a transition region and by a saddle-point transition state are reported, and comparison with theory is made.
A. H. Zewail, Faraday Discuss. Chem. Soc., 1991, 91, 207 DOI: 10.1039/DC9919100207
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