To understand mass transport at surfaces, a macroscopic theory is advanced based on the Onsager approach to non-equilibrium thermodynamics. A microscopic basis is then sought by re-examining the kinetic lattice-gas model to generalize the underlying dynamics for adsorption, desorption and diffusion.
H. J. Kreuzer, J. Chem. Soc., Faraday Trans., 1990, 86, 1299 DOI: 10.1039/FT9908601299
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