Herein we report for the first time on the gram-scale synthesis of a four-arm cage-shaped poly(ethylene oxide) (PEO) and its pioneering application as polymer electrolyte. The well-supressed crystallization by the cage architecture proves the great toolbox of polymer chemists to overcome crystallization issues in PEO-based polymer electrolytes.
A. J. Butzelaar, M. Gauthier-Jaques, K. L. Liu, G. Brunklaus, M. Winter and P. Theato, Polym. Chem., 2021, 12, 4326 DOI: 10.1039/D1PY00490E
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