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Optical Performance Improvement in Hydrothermal ZnO/Graphene Structure for Ultraviolet Lasing

Abstract

Ever since the exploration of ZnO for ultraviolet (UV) lasers, realization of high performance lasing in hydrothermal samples is still a challenge due to the poor crytal quality. In this paper, high quality ZnO microcavities were fabricated by hydrothermal method with graphene as grown media. Structural, optical as well as the exciton dynamic properties were studied systematically. Compared with the one grown without graphene, structured cavity morphology, higher light emission intensity and faster exciton recombination dynamics process were observed for ZnO grown on graphene, which makes the ZnO samples suitable for lasing. When it was excited by 325 nm femtosecond laser, single mode lasing with central wavelength about 393.2 and Q value about 936 was realized in a vertical cavity. If further increasing the exciton recombination rate through Al decoration, intensity improved multimode lasing was realzied. Our results propose a strategy for yielding single mode lasers in several micrometers with improved performances.

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Publication details

The article was received on 22 Dec 2017, accepted on 05 Feb 2018 and first published on 05 Feb 2018


Article type: Paper
DOI: 10.1039/C7TC05880B
Citation: J. Mater. Chem. C, 2018, Accepted Manuscript
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    Optical Performance Improvement in Hydrothermal ZnO/Graphene Structure for Ultraviolet Lasing

    F. Qin, C. Xu, Q. Zhu, J. Lu, F. Chen, D. You, Z. Zhu and A. G. Manohari, J. Mater. Chem. C, 2018, Accepted Manuscript , DOI: 10.1039/C7TC05880B

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