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A well-organized graphene nanostructure for versatile strain-sensing application constructed by a covalently bonded graphene/rubber interface

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Abstract

Graphene/rubber nanocomposites have attracted increasing attention for their fantastic applications in varied wearable electronics. However, the mechanical and functional properties of graphene/rubber nanocomposites are often limited by their weak interfacial interactions, such as ionic and hydrogen bonding. Here, we propose a covalently bonded graphene/rubber nanocomposite with a well-organized graphene nanostructure for versatile strain-sensing applications. Briefly, biological phytic acid was chosen as a covalent-bonding bridge to co-crosslink graphene oxide nanosheets and epoxidized natural rubber chains via the ring-opening reaction of epoxy groups. Benefiting from the covalently bonded interface, the obtained nanocomposite exhibited dramatically enhanced mechanical properties. Compared with the sulfur-cured sample, the tensile strength and elongation at break increased by 67.43% and 116.55%, respectively. Moreover, the covalent linkage facilitates the formation of a well-organized graphene network, which remarkably enhances the sensitivity and stability of the as-prepared strain sensors. The resultant sensors can monitor both large-scale and tiny human motion and exhibit great potential in the application of sign language recognition. This covalently bonded graphene/rubber interface opens the door to tailored design and low-cost fabrication of well-organized graphene nanostructures for multifunctional applications in electronic sensors, electromagnetic shielding materials, actuators for artificial muscles, etc.

Graphical abstract: A well-organized graphene nanostructure for versatile strain-sensing application constructed by a covalently bonded graphene/rubber interface

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Publication details

The article was received on 15 Dec 2017, accepted on 26 Jan 2018 and first published on 26 Jan 2018


Article type: Paper
DOI: 10.1039/C7TC05758J
Citation: J. Mater. Chem. C, 2018, Advance Article
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    A well-organized graphene nanostructure for versatile strain-sensing application constructed by a covalently bonded graphene/rubber interface

    Q. Guo, Y. Luo, J. Liu, X. Zhang and C. Lu, J. Mater. Chem. C, 2018, Advance Article , DOI: 10.1039/C7TC05758J

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