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A Flexible Rechargeable Zinc-Ion Wire-shaped Battery with Shape Memory Function

Abstract

The ever-growing development of flexible and wearable electronics boosts the research on flexible and wearable energy storage devices. However, those devices are susceptible to mechanical deformation, leading to inevitable damage and degradation of performances. Herein, we report the fabrication of a smart wire-shaped flexible and rechargeable Zn-ion battery with shape memory function, which enables the battery to restore the shape and energy storage capability against mechanical deformation by temperature triggered shape memory effect. As an energy storage device, the flexible wire battery delivered a discharging specific capacity of 143.2 mAh g-1 at 1 C in aqueous electrolyte and a significantly enhanced cyclic life due to the polypyrrole coating on the MnO2 nanocrystallines. Moreover, the performance was well-retained in a polymer gel electrolyte, delivered a discharge specific capacity of 135.2 mAh g-1 at 1 C and long cyclic stability over 1000 cycles, which could be attributed to the enhanced ionic conductivity and water retention properties offered by the gelatin-borax-based polymeric gel. Additionally, the intriguing mechanical properties of the Nitinol wire endowed the yarn battery with high flexibility upon bending and could recover the deformation by immersing in 45 oC water for multiple times while preserving the electrochemical performances.

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Publication details

The article was received on 04 Feb 2018, accepted on 05 Apr 2018 and first published on 05 Apr 2018


Article type: Paper
DOI: 10.1039/C8TA01172A
Citation: J. Mater. Chem. A, 2018, Accepted Manuscript
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    A Flexible Rechargeable Zinc-Ion Wire-shaped Battery with Shape Memory Function

    Z. Wang, Z. Ruan, Z. Liu, Y. Wang, Z. Tang, H. Li, M. Zhu, T. F. Hung, J. Liu, Z. Shi and C. Zhi, J. Mater. Chem. A, 2018, Accepted Manuscript , DOI: 10.1039/C8TA01172A

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