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Clustering and assembly dynamics of a one-dimensional microphase former

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Abstract

Both ordered and disordered microphases ubiquitously form in suspensions of particles that interact through competing short-range attraction and long-range repulsion (SALR). While ordered microphases are more appealing materials targets, understanding the rich structural and dynamical properties of their disordered counterparts is essential to controlling their mesoscale assembly. Here, we study the disordered regime of a one-dimensional (1D) SALR model, whose simplicity enables detailed analysis by transfer matrices and Monte Carlo simulations. We first characterize the signature of the clustering process on macroscopic observables, and then assess the equilibration dynamics of various simulation algorithms. We notably find that cluster moves markedly accelerate the mixing time, but that event chains are of limited help in the clustering regime. These insights will inspire further study of three-dimensional microphase formers.

Graphical abstract: Clustering and assembly dynamics of a one-dimensional microphase former

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Publication details

The article was received on 13 Feb 2018, accepted on 12 Mar 2018 and first published on 12 Mar 2018


Article type: Paper
DOI: 10.1039/C8SM00315G
Citation: Soft Matter, 2018, Advance Article
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    Clustering and assembly dynamics of a one-dimensional microphase former

    Y. Hu and P. Charbonneau, Soft Matter, 2018, Advance Article , DOI: 10.1039/C8SM00315G

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