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Autophoretic motion in three dimensions


Janus particles with the ability to move phoretically in self-generated chemical concentration gradients are model systems for active matter. Their motion typically consists of straight paths with rotational diffusion being the dominant reorientation mechanism. In this paper, we show theoretically that by a suitable surface coverage of both activity and mobility, translational and rotational motion can be induced arbitrarily in three dimensions. The resulting trajectories are in general helical, and their pitch and radius can be controlled by adjusting the angle between the translational and angular velocity. Building on the classical mathematical framework for axisymmetric self-phoretic motion under fixed-flux chemical boundary condition, we first show how to calculate the most general three-dimensional motion for an arbitrary surface coverage of a spherical particle. After illustrating our results on surface distributions, we next introduce a simple intuitive patch model to serve as a guide for designing arbitrary phoretic spheres.

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Publication details

The article was received on 26 Jan 2018, accepted on 08 Mar 2018 and first published on 08 Mar 2018

Article type: Paper
DOI: 10.1039/C8SM00194D
Citation: Soft Matter, 2018, Accepted Manuscript
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    Autophoretic motion in three dimensions

    M. K. Lisicki, S. Reigh and E. Lauga, Soft Matter, 2018, Accepted Manuscript , DOI: 10.1039/C8SM00194D

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