Robust mesoporous bimetallic yolk–shell catalysts for chemical CO2 upgrading via dry reforming of methane

Cameron-Alexander Hurd Price; Laura Pastor-Pérez; Tomas Ramirez Reina; Jian Liu

doi:10.1039/C8RE00058A

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Robust mesoporous bimetallic yolk–shell catalysts for chemical CO₂ upgrading via dry reforming of methane†

Cameron-Alexander Hurd Price,

^a Laura Pastor-Pérez,

^ab Tomas Ramirez Reina

*^a and Jian Liu

*^ac

Author affiliations

* Corresponding authors

^a Department of Chemical Engineering and Process Engineering, University of Surrey, Guildford, UK
E-mail: t.ramirezreina@surrey.ac.uk, jian.liu@surrey.ac.uk

^b Laboratorio de Materiales Avanzados, Departamento de Química Inorgánica – Instituto Universitario de Materiales de Alicante Universidad de Alicante, Apartado 99, E-03080 Alicante, Spain

^c State Key Laboratory of Catalysis, Dalian Institute of Chemical Physics, Chinese Academy of Sciences, 457 Zhongshan Road, Dalian 116023, China

Abstract

Here, we report the synthesis of mesoporous ZnO/Ni@m-SiO₂ yolk–shell particles. The unique ZnO/Ni@m-SiO₂ catalysts demonstrate impressive resistance to sintering and coking for dry reforming of methane (DRM). They also display long term stability with high levels of conversion and selectivity, making this catalyst promising for chemical CO₂ upgrading.

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Article information

DOI: https://doi.org/10.1039/C8RE00058A
Article type: Communication
Submitted: 10 Apr 2018
Accepted: 23 May 2018
First published: 19 Jun 2018
This article is Open Access

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React. Chem. Eng., 2018,3, 433-436

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Robust mesoporous bimetallic yolk–shell catalysts for chemical CO₂ upgrading via dry reforming of methane

C. H. Price, L. Pastor-Pérez, T. Ramirez Reina and J. Liu, React. Chem. Eng., 2018, 3, 433 DOI: 10.1039/C8RE00058A

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Reaction Chemistry & Engineering