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Facile synthesis of carbo- and heterocycles via Fe(III)-catalyzed alkene hydrofunctionalization

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Abstract

A facile synthesis of carbo- and heterocycles via Fe(III)-catalyzed alkene hydrofunctionalization has been developed. Various alkenes bearing a leaving group could convert to alkyl radicals through hydrogen atom transfer (HAT), and then serve as cyclization dipoles for accessing carbo- and heterocycles. The synthetic utility was further demonstrated by the synthesis of tetracyclic carbocycles from isopregol.

Graphical abstract: Facile synthesis of carbo- and heterocycles via Fe(iii)-catalyzed alkene hydrofunctionalization

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Publication details

The article was received on 09 Sep 2017, accepted on 30 Sep 2017 and first published on 10 Oct 2017


Article type: Research Article
DOI: 10.1039/C7QO00817A
Citation: Org. Chem. Front., 2018, Advance Article
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    Facile synthesis of carbo- and heterocycles via Fe(III)-catalyzed alkene hydrofunctionalization

    J. Qi, J. Zheng and S. Cui, Org. Chem. Front., 2018, Advance Article , DOI: 10.1039/C7QO00817A

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