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Copper-catalysed dehydrogenative α-C(sp3)–H amination of tetrahydroquinolines with O-benzoyl hydroxylamines

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Abstract

A copper-catalysed dehydrogenative α-C(sp3)–H amination of tetrahydroquinolines with O-benzoyl hydroxylamines has been demonstrated for the first time, which proceeds with the merits of operational simplicity, good functional tolerance, mild conditions, the use of O2 as the oxidant and no need for the installation of directing groups.

Graphical abstract: Copper-catalysed dehydrogenative α-C(sp3)–H amination of tetrahydroquinolines with O-benzoyl hydroxylamines

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Publication details

The article was received on 04 Sep 2017, accepted on 11 Oct 2017 and first published on 12 Oct 2017


Article type: Research Article
DOI: 10.1039/C7QO00794A
Citation: Org. Chem. Front., 2018, Advance Article
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    Copper-catalysed dehydrogenative α-C(sp3)–H amination of tetrahydroquinolines with O-benzoyl hydroxylamines

    H. Zhao, X. Chen, H. Jiang and M. Zhang, Org. Chem. Front., 2018, Advance Article , DOI: 10.1039/C7QO00794A

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