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Multicomponent Metal-Organic Frameworks Derivatives for Optimizing the Selective Catalytic Performance of Styrene Epoxidation Reaction

Abstract

Multicomponent metal-organic frameworks (MOFs) derivatives have attracted strong interest in energy and environmental fields. However, most of the papers focus on single MOFs derivatives, reports on multicomponent MOFs derivatives and their catalytic studies are relatively few. Here, we report an easy-to-operate strategy to obtain multicomponent MOFs derivatives by treating multicomponent MOFs under suitable gas atmosphere and high temperature. We use ZIF-67 as the template to introduce Zn and successfully obtain the multicomponent MOFs. After carbonization, the multicomponent MOFs derivatives with Co and CoO nanoparticles exhibit higher conversion of styrene (≈ 99%), higher selectivity (≈ 70%) and better stability than those of MOFs and the single component MOF derivative.

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Publication details

The article was received on 14 Feb 2018, accepted on 04 Apr 2018 and first published on 13 Apr 2018


Article type: Paper
DOI: 10.1039/C8NR01336E
Citation: Nanoscale, 2018, Accepted Manuscript
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    Multicomponent Metal-Organic Frameworks Derivatives for Optimizing the Selective Catalytic Performance of Styrene Epoxidation Reaction

    J. Hui, H. Chu, W. Zhang, Y. Shen, W. Chen, Y. Hu, W. Liu, C. Gao, S. Guo, G. Xiao, S. Li, Y. Fu, D. Fan, W. Zhang and F. Huo, Nanoscale, 2018, Accepted Manuscript , DOI: 10.1039/C8NR01336E

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