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Issue 2, 2018
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The reduction of 4-nitrophenol and 2-nitroaniline by the incorporation of Ni@Pd MNPs into modified UiO-66-NH2 metal–organic frameworks (MOFs) with tetrathia-azacyclopentadecane

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Abstract

We have found that UiO-66-NH2 can be used as an excellent support for the synthesis of highly sparse nanoparticles. UiO-66-NH2 has a high surface area that was functionalized with tetrathia-azacyclopentadecane (TTACP) groups acting as strong conjugation sites so that Ni@Pd nanoparticles were well dispersed without aggregation on the structures of the UiO-66-NH2 microspheres (UiO-66-NH2/TTACP/Ni@Pd). The synthesized UiO-66-NH2/TTACP/Ni@Pd magnetic nanoparticles (MNPs) exhibited excellent catalytic activity for the reduction of 2-nitroaniline and 4-nitrophenol.

Graphical abstract: The reduction of 4-nitrophenol and 2-nitroaniline by the incorporation of Ni@Pd MNPs into modified UiO-66-NH2 metal–organic frameworks (MOFs) with tetrathia-azacyclopentadecane

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Publication details

The article was received on 29 Sep 2017, accepted on 04 Dec 2017 and first published on 13 Dec 2017


Article type: Paper
DOI: 10.1039/C7NJ03732E
Citation: New J. Chem., 2018,42, 988-994
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    The reduction of 4-nitrophenol and 2-nitroaniline by the incorporation of Ni@Pd MNPs into modified UiO-66-NH2 metal–organic frameworks (MOFs) with tetrathia-azacyclopentadecane

    S. M. Sadeghzadeh, R. Zhiani and S. Emrani, New J. Chem., 2018, 42, 988
    DOI: 10.1039/C7NJ03732E

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