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Highly-Functionalized Arene Synthesis Based on Palladium on Carbon-Catalyzed Aqueous Dehydrogenation of Cyclohexadienes and Cyclohexenes

Abstract

The transition metal-catalyzed dehydrogenation is a clean oxidation method requiring no additional oxidant. We have accomplished an easily-removed Pd/C-catalyzed aqueous dehydrogenation of 1,4-cyclohexadienes and cyclohexenes to give the corresponding highly-functionalized arenes. Furthermore, the various arenes could be efficiently constructed in a one-pot manner via Diels-Alder reaction and the following dehydrogenation.

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Publication details

The article was received on 22 Dec 2017, accepted on 09 Feb 2018 and first published on 09 Feb 2018


Article type: Communication
DOI: 10.1039/C7GC03819D
Citation: Green Chem., 2018, Accepted Manuscript
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    Highly-Functionalized Arene Synthesis Based on Palladium on Carbon-Catalyzed Aqueous Dehydrogenation of Cyclohexadienes and Cyclohexenes

    N. Yasukawa, H. Yokoyama, M. Masuda, Y. Monguchi, H. Sajiki and Y. Sawama, Green Chem., 2018, Accepted Manuscript , DOI: 10.1039/C7GC03819D

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