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Issue 6, 2018
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Highly-functionalized arene synthesis based on palladium on carbon-catalyzed aqueous dehydrogenation of cyclohexadienes and cyclohexenes

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Abstract

Transition metal-catalyzed dehydrogenation is a clean oxidation method requiring no additional oxidants. We have accomplished a heterogeneous Pd/C-catalyzed aqueous dehydrogenation of 1,4-cyclohexadienes and cyclohexenes to give the corresponding highly-functionalized arenes. Furthermore, various arenes could be efficiently constructed in a one-pot manner via a Diels–Alder reaction and the following dehydrogenation.

Graphical abstract: Highly-functionalized arene synthesis based on palladium on carbon-catalyzed aqueous dehydrogenation of cyclohexadienes and cyclohexenes

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Publication details

The article was received on 22 Dec 2017, accepted on 09 Feb 2018 and first published on 09 Feb 2018


Article type: Communication
DOI: 10.1039/C7GC03819D
Citation: Green Chem., 2018,20, 1213-1217
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    Highly-functionalized arene synthesis based on palladium on carbon-catalyzed aqueous dehydrogenation of cyclohexadienes and cyclohexenes

    N. Yasukawa, H. Yokoyama, M. Masuda, Y. Monguchi, H. Sajiki and Y. Sawama, Green Chem., 2018, 20, 1213
    DOI: 10.1039/C7GC03819D

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