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A novel route with a Cu(II)-MOF-derived structure to synthesize Cu/Cu2O NPs@graphene: the electron transfer leads to the synergistic effect of the Cu(0)–Cu(I) phase for an effective catalysis of the Sonogashira cross-coupling reactions

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Abstract

A uniformly dispersed two-phase Cu/Cu2O NPs@graphene was obtained via an innovative “take” and “off” synthesis strategy with a Cu-MOF-derived jacket structure. The electron transfer between the Cu phase and Cu2O phase leads to the synergistic effect of the Cu(0)–Cu(I) phase for an efficient catalysis of the Sonogashira cross-coupling reactions.

Graphical abstract: A novel route with a Cu(ii)-MOF-derived structure to synthesize Cu/Cu2O NPs@graphene: the electron transfer leads to the synergistic effect of the Cu(0)–Cu(i) phase for an effective catalysis of the Sonogashira cross-coupling reactions

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Publication details

The article was received on 03 Feb 2018, accepted on 25 Mar 2018 and first published on 26 Mar 2018


Article type: Communication
DOI: 10.1039/C8DT00465J
Citation: Dalton Trans., 2018, Advance Article
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    A novel route with a Cu(II)-MOF-derived structure to synthesize Cu/Cu2O NPs@graphene: the electron transfer leads to the synergistic effect of the Cu(0)–Cu(I) phase for an effective catalysis of the Sonogashira cross-coupling reactions

    W. Sun, L. Gao, X. Sun and G. Zheng, Dalton Trans., 2018, Advance Article , DOI: 10.1039/C8DT00465J

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