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High selectivity of CO2 hydrogenation to CO by controlling the valence state of nickel using perovskite

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Abstract

The selectivity of CO2 hydrogenation can be significantly tuned by controlling the valence state of nickel using lanthanum–iron–nickel perovskites. Nickel with higher valence states weakens the binding of CO and increases the activation barrier for further CO hydrogenation, leading to a higher CO selectivity than the metallic nickel.

Graphical abstract: High selectivity of CO2 hydrogenation to CO by controlling the valence state of nickel using perovskite

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Publication details

The article was received on 12 May 2018, accepted on 10 Jun 2018 and first published on 11 Jun 2018


Article type: Communication
DOI: 10.1039/C8CC03829E
Citation: Chem. Commun., 2018, Advance Article
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    High selectivity of CO2 hydrogenation to CO by controlling the valence state of nickel using perovskite

    B. Zhao, B. Yan, Z. Jiang, S. Yao, Z. Liu, Q. Wu, R. Ran, S. D. Senanayake, D. Weng and J. G. Chen, Chem. Commun., 2018, Advance Article , DOI: 10.1039/C8CC03829E

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