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From open-shell singlet diradicaloids to polyradicaloids

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Abstract

In this Feature Article, we highlight our recent efforts toward stable open-shell singlet diradicaloids and polyradicaloids. A brief review on the historical works in the area is introduced first, followed by discussion on the fundamental electronic and physical properties of open-shell singlet diradicaloids. Then, the structure–diradical character relationships based on our recently developed diradicaloids are presented. Next, the challenges and solutions toward stable polyradicaloids and 3D π-conjugated diradicaloids are discussed. Finally, their preliminary material applications are introduced and a perspective view of the area is given.

Graphical abstract: From open-shell singlet diradicaloids to polyradicaloids

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Publication details

The article was received on 30 Dec 2017, accepted on 31 Jan 2018 and first published on 31 Jan 2018


Article type: Feature Article
DOI: 10.1039/C7CC09949E
Citation: Chem. Commun., 2018, Advance Article
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    From open-shell singlet diradicaloids to polyradicaloids

    T. Y. Gopalakrishna, W. Zeng, X. Lu and J. Wu, Chem. Commun., 2018, Advance Article , DOI: 10.1039/C7CC09949E

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