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An imidazolium-functionalized mesoporous cationic metal–organic framework for cooperative CO2 fixation into cyclic carbonate

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Abstract

A mesoporous cationic Cr-MOF, termed FJI-C10, containing imidazolium moieties, Lewis acidic Cr3+ sites and free halogens is constructed for the first time by a topology-guided one-pot synthesis. FJI-C10 exhibits excellent performances in CO2 adsorption (20.2 wt% at 273 K and 1 bar) and chemical fixation of CO2 into cyclic carbonates without the use of co-catalyst under atmospheric pressure.

Graphical abstract: An imidazolium-functionalized mesoporous cationic metal–organic framework for cooperative CO2 fixation into cyclic carbonate

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Publication details

The article was received on 09 Nov 2017, accepted on 21 Nov 2017 and first published on 21 Nov 2017


Article type: Communication
DOI: 10.1039/C7CC08630J
Citation: Chem. Commun., 2018, Advance Article
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    An imidazolium-functionalized mesoporous cationic metal–organic framework for cooperative CO2 fixation into cyclic carbonate

    J. Liang, Y. Xie, X. Wang, Q. Wang, T. Liu, Y. Huang and R. Cao, Chem. Commun., 2018, Advance Article , DOI: 10.1039/C7CC08630J

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