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A facile method to construct a 2,4,9-triazaadamantane skeleton and synthesize nitramine derivatives

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Abstract

An unusual protocol for a “one-pot” three-step reaction to build a 2,4,9-triazaadamantane skeleton from triallylcarbinol was developed. The design and execution of these tactics are described in detail. Then a novel high energy density compound 2,4,9-trinitro-2,4,9-triazaadamantane-7-yl nitrate was prepared and fully characterized. The results indicate that this compound exhibits high thermal stability and high density (1.840 g cm−3).

Graphical abstract: A facile method to construct a 2,4,9-triazaadamantane skeleton and synthesize nitramine derivatives

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Publication details

The article was received on 05 May 2017, accepted on 12 Jun 2017 and first published on 13 Jun 2017


Article type: Research Article
DOI: 10.1039/C7QO00357A
Citation: Org. Chem. Front., 2017, Advance Article
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    A facile method to construct a 2,4,9-triazaadamantane skeleton and synthesize nitramine derivatives

    T. Hou, J. Zhang, C. Wang and J. Luo, Org. Chem. Front., 2017, Advance Article , DOI: 10.1039/C7QO00357A

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