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Issue 7, 2017
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A bifunctional covalent organic framework as an efficient platform for cascade catalysis

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Abstract

A bifunctional covalent organic framework (COF) has been illustrated in the context of partial metalation of a highly porous and chemically robust pyridine containing COF (COF-TpPa-Py) with Pd species and by taking advantage of the base catalytic behavior of pyridine. The resultant bifunctionalized COF exhibits excellent performance in catalyzing one-pot cascade aerobic oxidation–Knoevenagel condensation reactions, outperforming the corresponding homogeneous and porous organic polymer based catalytic systems, thereby opening a new avenue for multifunctional COFs as a promising platform for heterogeneous cascade catalysis.

Graphical abstract: A bifunctional covalent organic framework as an efficient platform for cascade catalysis

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Publication details

The article was received on 15 Dec 2016, accepted on 22 Jan 2017 and first published on 23 Jan 2017


Article type: Research Article
DOI: 10.1039/C6QM00363J
Citation: Mater. Chem. Front., 2017,1, 1310-1316
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    A bifunctional covalent organic framework as an efficient platform for cascade catalysis

    Q. Sun, B. Aguila and S. Ma, Mater. Chem. Front., 2017, 1, 1310
    DOI: 10.1039/C6QM00363J

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