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Issue 14, 2017
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Manganese(III) acetate catalyzed oxidative amination of benzylic C(sp3)–H bonds with nitriles

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Abstract

Mn-Catalyzed oxidative amination of benzylic C(sp3)–H bonds with nitriles is disclosed, which enables the synthesis of a broad range of secondary amides in moderate to excellent yields under mild conditions. The interaction between Mn(III) and DDQ facilitates the oxidation and makes it highly efficient and selective.

Graphical abstract: Manganese(iii) acetate catalyzed oxidative amination of benzylic C(sp3)–H bonds with nitriles

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Publication details

The article was received on 01 Mar 2017, accepted on 09 Mar 2017 and first published on 09 Mar 2017


Article type: Communication
DOI: 10.1039/C7OB00512A
Citation: Org. Biomol. Chem., 2017,15, 2897-2901
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    Manganese(III) acetate catalyzed oxidative amination of benzylic C(sp3)–H bonds with nitriles

    Y. Zhang, J. Dong, L. Liu, L. Liu, Y. Zhou and S. Yin, Org. Biomol. Chem., 2017, 15, 2897
    DOI: 10.1039/C7OB00512A

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