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Issue 11, 2017
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Chemically and physically robust, commercially-viable iron-based composite oxygen carriers sustainable over 3000 redox cycles at high temperatures for chemical looping applications

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Abstract

High attrition of oxygen carriers from ionic diffusion induced morphological changes is one of the most serious obstacles inhibiting commercialization of chemical looping processes. By confining active oxygen carriers in an Al-based skeleton, a low-cost oxygen carrier achieving high chemical and physical stability over 3000 TGA redox cycles with exceptional attrition resistance and reactivity in a high pressure and temperature, chemical looping moving bed pilot plant, is enabled for commercial implementation.

Graphical abstract: Chemically and physically robust, commercially-viable iron-based composite oxygen carriers sustainable over 3000 redox cycles at high temperatures for chemical looping applications

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Publication details

The article was received on 16 Sep 2017, accepted on 13 Oct 2017 and first published on 13 Oct 2017


Article type: Communication
DOI: 10.1039/C7EE02657A
Citation: Energy Environ. Sci., 2017,10, 2318-2323
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    Chemically and physically robust, commercially-viable iron-based composite oxygen carriers sustainable over 3000 redox cycles at high temperatures for chemical looping applications

    C. Chung, L. Qin, V. Shah and L. Fan, Energy Environ. Sci., 2017, 10, 2318
    DOI: 10.1039/C7EE02657A

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