Building premium secondary reaction field with a miniaturized capsule catalyst to realize efficient synthesis of a liquid fuel directly from syngas

Noriyuki Yamane; Yang Wang; Jie Li; Yingluo He; Peipei Zhang; Letrunghieu Nguyen; Li Tan; Peipei Ai; Xiaobo Peng; Ye Wang; Guohui Yang; Noritatsu Tsubaki

doi:10.1039/C7CY00224F

Building premium secondary reaction field with a miniaturized capsule catalyst to realize efficient synthesis of a liquid fuel directly from syngas†

Noriyuki Yamane,^ab Yang Wang,

^a Jie Li,^a Yingluo He,^a Peipei Zhang,^a Letrunghieu Nguyen,^a Li Tan,^a Peipei Ai,^a Xiaobo Peng,*^a Ye Wang,

^c Guohui Yang*^a and Noritatsu Tsubaki

*^a

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^a Department of Applied Chemistry, School of Engineering, University of Toyama, Gofuku 3190, Toyama 930-8555, Japan
E-mail: hhpengxiaobo@hotmail.com, thomas@eng.u-toyama.ac.jp, tsubaki@eng.u-toyama.ac.jp

^b Research & Development, Nippon Steel & Sumitomo Metal Corporation, 20-1 Shintomi, Futtsu, Chiba 293-8511, Japan

^c State Key Laboratory of Physical Chemistry of Solid Surfaces, College of Chemistry and Chemical Engineering, Xiamen University, Xiamen 361005, China

Abstract

Herein, we report a new miniaturized capsule catalyst, Co/SiO₂-M-Z_6ET, which is different from routine capsule catalysts, has a smaller core size and has stronger Brønsted acidity. The premium secondary reaction field and the significant capsule size effect on Co/SiO₂-M-Z_6ET were demonstrated using a model compound of n-hexadecane (n-C₁₆). Furthermore, a striking gasoline selectivity of 72% was facilely obtained from FT synthesis.

Catalysis Science & Technology

Building premium secondary reaction field with a miniaturized capsule catalyst to realize efficient synthesis of a liquid fuel directly from syngas†

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Building premium secondary reaction field with a miniaturized capsule catalyst to realize efficient synthesis of a liquid fuel directly from syngas

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